Abstract
We demonstrate site-resolved imaging of individual bosonic atoms in a Hubbard-regime two-dimensional optical lattice with a short lattice constant of 266 nm. To suppress the heating by probe light with the 1S0–1P1 transition of the wavelength λ = 399 nm for high-resolution imaging and preserve atoms at the same lattice sites during the fluorescence imaging, we simultaneously cool atoms by additionally applying narrow-line optical molasses with the 1S0–3P1 transition of the wavelength λ = 556 nm. We achieve a low temperature of , corresponding to a mean oscillation quantum number along the horizontal axes of 0.22(4) during the imaging process. We detect, on average, 200 fluorescence photons from a single atom within a 400 ms exposure time, and estimate a detection fidelity of 87(2)%. The realization of a quantum gas microscope with enough fidelity for Yb atoms in a Hubbard-regime optical lattice opens up the possibilities for studying various kinds of quantum many-body systems such as Bose and Fermi gases, and their mixtures, and also long-range-interacting systems such as Rydberg states.
Export citation and abstract BibTeX RIS
Original content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence. Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI.
1. Introduction
Ultracold quantum gases in optical lattices have proven extremely useful for the study of quantum phases and the dynamical evolutions of strongly correlated many-body system described by a Hubbard model [1]. Well-known examples include a quantum phase transition from a superfluid (SF) to a Mott insulator (MI) for bosonic species [2–4], and a crossover from a metal to a MI for fermionic species [5, 6]. To fully exploit the potential of ultracold atoms in an optical lattice as a quantum simulator, it is a great advantage to have access to the in-trap atom distribution with single-atom resolution. In 2009, a quantum gas microscope (QGM) was realized with bosonic for the first time [7]. Site-resolved imaging has been used to study the SF to MI transition [8, 9], and strongly correlated dynamics in optical lattices [10–12]. Site-resolved imaging systems have been realized for other alkaline atomic species such as fermionic [13–15] and [16–18] very recently.
Extending the applicability of a QGM technique to atomic species beyond alkali-metal atoms is an important step for a further revolution. In particular, a successful application of a QGM technique to two-electron atoms such as alkaline-earth metal and ytterbium (Yb) atoms is remarkable because it offers many unique possibilities for quantum simulation and quantum information research. In fact, recent studies demonstrate that a system of two-electron atoms in an optical lattice is an ideal platform for the study of SU() physics [19–22], two-orbital SU() physics [23–26], and topological physics [27]. In addition, a variety of stable isotopes, 5 bosonic and 2 fermionic isotopes in the case of Yb atoms for example, enable us to study various kinds of many-body systems such as ultracold Bose and Fermi gases and Bose–Bose [28, 29], Bose–Fermi [29–31], and Fermi–Fermi [20] mixtures in an optical lattice. The existence of nuclear spin degrees of freedom in the ground state 1S0 and long-lived metastable states 3P0 and 3P2 offers unique possibilities for quantum memory and quantum computation [32–35]. Additionally we can tune interatomic interactions between the 1S0 and 3P2 states by an anisotropy-induced magnetic Feshbach resonance [36]. Furthermore, a high-resolution laser spectroscopy of atoms in an optical lattice using the ultranarrow 1S0-3P0 and 1S0-3P2 optical transitions is also demonstrated both for bosons and fermions, revealing the novel behaviour of the atomic interaction of the system [24–26, 36, 37]. There has been also considerable interest in high-lying Rydberg states of two-electron atoms [38, 39] in an optical lattice [40] because of an additional degrees of freedom for probing and manipulation provided by the remaining valence electron of a singly excited Rydberg state. The successful application of a QGM technique to these systems will definitely enhance our understanding of the physics described in the above.
The important progress towards this direction has been reported quite recently in [41], in which a site-resolved imaging system has been realized without cooling process for atoms in a two-dimensional (2D) optical lattice with a lattice constant of 544 nm. The achieved resolution of ∼310 nm (full width at half maximum, FWHM) is impressively small. A further study is still necessary, however, to successfully perform the above mentioned interesting researches for Yb atoms using a QGM. First, a crucial aspect of QGM is the high-fidelity of the imaging process characterized by loss and hopping rates during the fluorescence imaging, which should be evaluated by comparing two successive images taken for the same atoms. Second, the Hubbard-regime optical lattice needs a shorter lattice constant, especially for heavier atoms of Yb. These conditions should be simultaneously satisfied with the single-site resolved imaging and single-atom sensitivity.
In this work, we achieve site-resolved imaging of individual atoms in a 2D optical lattice with a short lattice constant of 266 nm which ensures the Hubbard-regime [42]. To keep atoms at the same lattice sites during the fluorescence imaging, we simultaneously cool atoms by additionally applying narrow-line optical molasses with the 1S0-3P1 transition (, the Doppler limit temperature , natural linewidth ), resulting in a low temperature of , corresponding to a mean oscillation quantum number along the horizontal axes 0.22(4) during imaging process (see figure 1(a) for relevant energy levels). In particular, the careful tuning of the relative angle between an applied magnetic field and a polarization of lattice laser beams realizes the cancellation of the inhomogeneity of the light-shifts, which enhances a cooling efficiency of narrow-line laser cooling, both for sideband cooling along the horizontal direction and Doppler cooling along the vertical direction. The realization of such high efficient cooling allows for the suppression of heating due to the probe light using the 1S0-1P1 transition (, the Doppler limit temperature , natural linewidth ) for high-resolution imaging (see figure 1(a)). We achieve a lifetime of atoms during fluorescence imaging much longer than a typical imaging time of 400 ms, enabling to take multiple images for the same atomic sample and to successfully estimate the imaging fidelity to be 87(2)%. The realization of a QGM with enough fidelity for Yb atoms in a Hubbard-regime optical lattice opens up the possibilities for studying various kinds of quantum many-body systems such as Bose and Fermi gases, and their mixtures in an optical lattice, and also long-range-interacting systems such as Rydberg states.
The paper is organized as follow. In section 2, we describe an experimental setup and a method for preparation of an atom sample in a 2D lattice system. Section 3 presents cooling mechanism for realization of a site-resolved imaging and section 4 shows the results of the analysis of site-resolved fluorescence images including loss and hopping rates. Finally we conclude our work with brief prospects in section 5.
2. Experimental setup and atom preparation
Our experiment starts from loading atoms into a magneto-optical trap (MOT) in a metal chamber and transferring the atoms into a glass cell (Schott AG BOROFLOAT) using an optical tweezer (OT). The detail of the MOT and OT setup is described in [43]. The position of atoms in the glass cell is about 5.5 mm below the surface of the glass cell, and just 6.23 mm under a high-resolution objective with numerical aperture of NA = 0.75 (Mitutoyo G Plan Apo HR50x (custom)), which is schematically shown in figure 1(b). After creating a Bose–Einstein condensate (BEC) of atoms after 10 s evaporative cooling in a crossed optical trap formed by the OT beam and another 532 nm beam, we load the BEC into a vertical lattice generated by the interference of two laser beams with the wavelength of propagating at a relative angle of . The vertical lattice has a spacing of and the trap frequency along the vertical axis (z-axis) of at this loading stage, as explained in detail in our previous work [44].
The atoms, just after being loaded into the vertical lattice, spread over several, typically three, layers, as shown in the left panel of figure 2(a). In this situation, although we can focus on the atoms in one selected layer with an objective depth of less than , we always have contributions from the atoms in other layers which considerably blur the image. To observe a clear image of the atoms in only one layer, we blow away the atoms in unnecessary layers. This is done by alternately exciting the atoms into the state under a bias magnetic field and a magnetic field gradient , corresponding to the Zeeman shift , followed by the rapid inelastic collisional decay and repumping back the atoms into the ground state (see figure 2(b)). Here the ultranarrow optical transition of 1S0- with the resonant wavelength of and natural linewidth is used for the excitation and -3S1 and 3P0-3S1 for repumping (see figure 2(c)). As a result, we successfully prepare the atoms in only a single layer, as shown in the right panel of figure 2(a).
Download figure:
Standard image High-resolution imageFinally, we load the 2D atom cloud in a single layer into horizontal 2D optical lattices (x- and y-axes) by simultaneously ramping up the potential of the vertical and horizontal optical lattices, where the wavelength of horizontal lattices is and the lattice spacing is . The vibrational frequencies along the three axes at the fluorescence imaging stage are , corresponding to the lattice depths of , respectively.
3. Narrow-line laser cooling in an optical lattice
An important prerequisite for realizing a QGM is to preserve the atoms at their sites during fluorescence imaging. The 1S0−1P1 transition provides high-resolution imaging with the diffraction limited resolution of a FWHM of 274 nm in our system. However, the high Doppler cooling limit temperature makes quite difficult to preserve atoms at their sites. In addition, the lack of hyperfine structure in the ground state 1S0 of bosonic Yb atom makes impossible to apply sub-Doppler cooling techniques such as polarization-gradient cooling and Raman sideband cooling. To resolve this difficulty, we simultaneously cool the atoms with Doppler and sideband cooling using the 1S0–3P1 narrow-line transition.
To efficiently cool all the atoms in an optical lattice with the narrow-line transition 1S0–3P1, we need to suppress the inhomogeneity of light shift between the 1S0 and 3P1 states, otherwise the detuning for cooling is not optimized simultaneously for all atoms. Here the light shift in the ground state 1S0 is given by , where I is the laser intensity of the wavelength and is the calculated scalar polarizability in the 1S0 state. The light shift in the magnetic sublevel of the 3P1 state is given as [45]
where
Here θ is the angle between the quantization axis and the polarization of laser beams, and are the scalar and tensor polarizabilities in the 3P1 state, respectively. Importantly, equation (2) provides the possibility of tuning the polarizability to coincide with by choosing an appropriate angle θ for mJ, thus canceling the light-shift effects of the 1S0–3P1 transition. For this possibility we perform a laser spectroscopy with the 1S0–3P1 transition for various laser intensities and angles θ, and accurately determine and as and , respectively. With these values, our current setup of the polarizations of all the lattice beams parallel to the vertical axis provides . In our experiment, however, we slightly tilt a magnetic field from the vertical direction by an angle which gives . This setup enables us to excite the atoms into the state, when the polarizations of the 556 nm cooling light along the horizontal axes are set to vertical, and those along the vertical axis horizontal (see figure 1(b)). Note that the light shift of the 1S0–1P1 transition for probing is smaller than the natural linewidth of this transition of 29 MHz, and so it is not a problem. The total intensities of 399 nm and 556 nm beams correspond to the saturation parameters of and , respectively. With this dual molasses, Moiré patterns of about 6 pitch are observed as a result of the interference between the cooling molasses beam of 556 nm and the optical lattice of 532 nm. To erase this unwanted Moiré pattern, we modulate the phase of the standing wave of the 556 nm optical molasses by modulating retro-reflecting mirrors via the attached Piezo transducers, as explained in detail in our previous work [44].
The fine tuning of the relative angle between a magnetic field and lattice laser polarizations indeed gives us a reasonably narrow resonance of the 1S0– transition for atoms in the optical lattice during fluorescence imaging. Figure 3(a) shows the spectra of atoms in our deepest horizontal optical lattices of , where is recoil energy of lattice beam. The top panel shows the fluorescence counts of 399 nm probe molasses light as a function of a frequency of 556 nm cooling molasses beams along the horizontal axes, in which we simultaneously apply the probe light and weak cooling molasses lights, and , and we can observe many fluorescence counts during a 400 ms exposure time only when the cooling is efficient at favorable detunings. We obtain the optimal frequency with the width of kHz (FWHM). The bottom panel shows the optical density measured by absorption imaging with a 556 nm beam irradiated along the horizontal axis as a function of a frequency of the 556 nm probe light. In this measurement we do not apply 399 and 556 nm molasses beams. Note that we set a zero frequency detuning as the resonance frequency of this spectrum. We determine the optimal detuning of cooling beam along the horizontal axes . The same measurements are done at several horizontal lattice depths, as shown in figure 3(b). In our lattice system, Lamb-Dicke parameters are , where k is a wavevector of 556 nm light, and . Although the frequency separation between the cooling sideband fR and the carrier transition f = 0, corresponding to the trap frequencies and , is not large enough compared with the natural linewidth of 184 kHz for the 556 nm cooling transition, as shown in figure 3(a), the responsible cooling mechanism along the x- and y-axes should be sideband cooling, because the optimal detuning of cooling beam along the horizontal axis depends on the horizontal lattice trap depth and is consistent with the trap frequency along the horizontal axis, as shown in figure 3(b). We note that the shape of the resonance dose not change for all the horizontal lattice potential depths of to studied in this measurement.
Download figure:
Standard image High-resolution imageThe temperature of the atoms during the fluorescence imaging is accurately measured by laser spectroscopy using the ultranarrow transition 1S0–. Figure 3(c) shows the spectrum obtained, which clearly shows three peaks corresponding to the red- and blue-sidebands and the main carrier. From the ratio of the red to the blue sideband peaks , we can evaluate a mean oscillation quantum number in a horizontal optical lattice , corresponding to the atomic temperature of [46–48]. The value is in agreement with the theoretical one of based on a sideband cooling theory [47]. Note that this expression is valid for a narrow enough laser linewidth compared to Γ and a low enough laser power that there is no need to consider a saturation effect. The temperature along the vertical direction is measured by a time-of-flight method to be 12(1) . The optimal detunings are determined for various lattice depths, and are independent of the lattice depth, which suggests that the dominant cooling mechanism is Doppler cooling. This is reasonable if we consider the small trap frequency of 15.7 kHz along the vertical direction compared with the linewidth of 184 kHz.
The unique feature of our scheme is the separation of the cooling and probing processes during the fluorescence imaging. We can therefore study the effect of the cooling beams alone. Here we study the temporal evolution of the temperature with narrow-line laser cooling, especially at the early stage of cooling, to investigate what happens during the cooling process. This is especially interesting because the atom loss rate for the light-assisted collision associated with the states is small [49] and the atoms in multiply-occupied sites would be heated without loss, differently from the case of alkali atoms. In this measurement, the temperature is measured by a time-of-flight method with absorption imaging. To correctly estimate the temperature along the horizontal axis, we numerically calculate the size of the atom cloud after a time-of-flight, assuming an initial Boltzman occupation of the each vibrational level and a ballistic expansion of the cloud. Figure 4(a) shows the results of the measurements. The temperatures rapidly increase within several milliseconds followed by the rather slow decrease towards the steady-state value obtained by the ultranarrow line laser spectroscopy of figure 3(c). This behaviour is explained as an effect of a light-assisted collision due to the near-resonant cooling light. Namely, atoms in multiply-occupied sites should be heated by release of the kinetic energy subsequent on a light-assisted collision. This is confirmed by further measurements with applying a photoassociation (PA) pulse for removal of multiply-occupied sites before imaging, shown in figure 4(b). In spite of the fluctuation of data, it is clear that the behaviour of the temperatures of figure 4(b) is different from that of figure 4(a). Although all the following single-site resolved imaging data presented in this paper are measured without the application of PA light, this initial heating effect is negligible because the multiply-occupied sites are almost absent in sparse atomic samples used for our QGM measurement.
Download figure:
Standard image High-resolution image4. Site-resolved imaging
We image the atomic fluorescence onto the EMCCD camera (Andor iXon Blue). In figure 5(a) we show one illustrative example of the obtained images. Note that, just before the fluorescence imaging, we intentionally select only about of the atoms for easier evaluation of the performance of the QGM. Such dilution of the atoms is done by performing a weak excitation with the 1S0– transition, and then returning the atoms back into the ground state 1S0. Figure 5(b) shows our measured point spread function (PSF), obtained by averaging over 104 fluorescence images of individual atoms. We find that our PSF can be well approximated by a double Gaussian:
with widths , main and relative amplitudes , a spatial offset r0, and an overall count offset C. The fit result shows our PSF is well described with nm and nm, and also has a FWHM of 364 nm, and we detect on average 200 photons per atom within 400 ms fluorescence time. In our imaging system, the spherical aberration remains, making the resolution of PSF worse than ideal one. Our system has a total fluorescence collection efficiency of 6.0%, given by the objective's solid angle of 17%, 51% total transmission through the imaging optics, and quantum efficiency of 70% of our EMCCD camera. The corresponding atomic fluorescence rate of ∼8300 photons/s is large enough to unambiguously identify the presence or absence of an atom for each lattice site. Note that the maximum number of detected photons is limited by the cooling rate of the narrow transition [44]. Although the resolution of measured PSF is about 1.4 times larger than the lattice spacing, we successfully determine the atomic distribution by deconvolution of images.
Download figure:
Standard image High-resolution imageFor reconstructing an atom distribution from our obtained images, we first determine a lattice angle and spacing from the isolated, single-site resolved signals [8]. Our lattice axes are oriented approximately along the vertical and horizontal axes with respect to the images. The histogram of the mutual distances in the coordination rotated by a small angle ϕ is shown in figure 5(c) and (d). We fit a periodic array of Gaussians to the observed histogram. Figure 5(e) shows the width of the Gaussians in the histogram as a function of a coordinate rotation angle. The red dotted line is a fit by . The minimum width of the histogram is obtained at the coordinate rotation angle of and the lattice constant of 2.66(1) pixels on CCD plane corresponding to the lattice constant of 266 nm. From the same analysis of the other lattice axis, we also obtain the coordinate rotation angle of and lattice constant of 2.65(1) pixels on CCD plane corresponding to the lattice constant of 266 nm. Thus, the magnification ratio of our imaging system is 159.7(4) and one pixel of our CCD camera corresponds to 100.2(3) nm on the objective plane. These values are used for the deconvolution analysis of our images. Figure 5(f) shows a raw image of the limited region of figure 5(a) with grid lines showing lattice separation and orientation. In figure 5(g), we show a reconstructed atom distribution where red circles and black dots represent the atoms and the lattice sites, respectively. In figure 5(h), we also show the reconstructed atom distribution convoluted with the model PSF of equation (3), which is compared with the raw image of figure 5(f).
An important aspect of QGM is the high-fidelity of the imaging process characterized by loss and hopping rates during the fluorescence imaging. For this purpose, we take two successive images of the same atoms with 400 ms exposure time and 300 ms delay between the two images, and observe the change in the distribution. We precisely tune the detuning of cooling molasses along the horizontal axes, and evaluate the loss and hopping rates during the fluorescence image from the two successive images. Figure 6(a) and (b) show the results of reconstructed atom distributions at , respectively. For optimized parameters, we achieve loss rates of 6.5(18)% and hopping rates of 6.7(15)% for 400 ms exposures of clouds with fillings of ∼0.02 (see figure 6(c)). These rates, which include reconstruction errors, give a detection fidelity of 87(2)% for sparse clouds. Here we discuss the origins of the measured loss and hopping rates. The thermal hopping cannot explain the observed rates since the average occupation number during the fluorescence imaging is as low as 0.22. Instead, several possible mechanisms can be considered such as the branching from the 1P1 to lower states [50], a vibrational quantum number-changing transition during the absorption and fluorescence cycle of the 1S0–1P1 transition, and the photon scattering from the 3P1 state due to the 532 nm lattice beams. The loss rate estimated with the lifetime about 10 s during fluorescence imaging is 6.8%. This value is in good agreement with the measured loss rate. We also note that one of the limiting factors of the lifetime is the irradiation of the 399 nm probe light itself.
Download figure:
Standard image High-resolution image5. Conclusion
In conclusion, we demonstrate a bosonic QGM for a 2D optical lattice with a short lattice constant of 266 nm. The atoms are preserved in the lattice sites during fluorescence imaging by narrow-line laser cooling which successfully combines Doppler cooling and sideband cooling. The resulting temperature is , corresponding to a mean oscillation quantum number along the horizontal axes 0.22(4). The PSF has a reasonably small width comparable to the ideal value, enabling the identification of the presence and absence of atoms by the deconvolution analysis. The high fidelity of the imaging process, which is an important aspect of QGM, is confirmed by the measurement of loss rate of 6.5(18)% and hopping rate of 6.7(15)% for 400 ms exposure time.
While we perform the experiment with bosonic atoms, our method is applicable for a QGM for other Yb isotopes, including fermionic and . In fact, our preliminary result shows that we can successfully obtain site-resolved images for fermionic atoms. In addition, the sideband cooling demonstrated in this work can be straightforwardly applied to other alkaline-earth atoms such as strontium, especially for an optical lattice with magic wavelength. The realization of a QGM with enough fidelity for Yb atoms in a Hubbard-regime optical lattice opens up the possibilities for studying various kinds of quantum many-body systems, and also long-range-interacting systems such as Rydberg states.
Acknowledgments
We would like to thank K Shibata for the setup of this experiment and T Fukuhara for useful discussions. This work was supported by the Grant-in-Aid for Scientific Research of JSPS (Nos. 13J00122, 25220711, 26247064, 26610121) and the Impulsing Paradigm Change through Disruptive Technologies (ImPACT) program.
Appendix. Deconvolution procedure
Here we describe the deconvolution procedure of our fluorescence image. First step is to determine a PSF, a lattice spacing, and a coordinate rotation angle from the isolated, single-site resolved signals, as is explained in detail in section 4. From the determined PSF of equation (3) and the location of lattice sites, we next calculate a trial image
where represents a position in an image plane, a position of a lattice site n, a fitting parameter corresponding to a probability of finding an atom at a lattice site n, and . Note that represents a fitted value of a peak fluorescence count at the n-th lattice site. Finally we determine the parameters by minimizing a quantity , where is a raw fluorescence image. As a typical example of this deconvolution procedure, we show in figure A1 a histogram of determined in several regions of 9 × 9 sites picked up from raw images.
Download figure:
Standard image High-resolution image