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Tensile Strength of Porous Dust Aggregates

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Published 2019 April 3 © 2019. The American Astronomical Society. All rights reserved.
, , Citation Misako Tatsuuma et al 2019 ApJ 874 159 DOI 10.3847/1538-4357/ab09f7

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0004-637X/874/2/159

Abstract

Comets are thought to have information about the formation process of our solar system. Recently, detailed information about comet 67P/Churyumov–Gerasimenko was found by Rosetta. It is remarkable that its tensile strength was estimated. In this paper, we measure and formulate the tensile strength of porous dust aggregates using numerical simulations, motivated by a porous dust aggregation model of planetesimal formation. We perform three-dimensional numerical simulations using a monomer interaction model with a periodic boundary condition. We stretch out a dust aggregate with a various initial volume filling factor between 10−2 and 0.5. We find that the tensile stress takes the maximum value at the time when the volume filling factor decreases to about half of the initial value. The maximum stress is defined to be the tensile strength. We take an average of the results with 10 different initial shapes to smooth out the effects of initial shapes of aggregates. Finally, we numerically obtain the relation between the tensile strength and the initial volume filling factor of dust aggregates. We also use a simple semi-analytical model and successfully reproduce the numerical results, which enables us to apply a wide parameter range and different materials. The obtained relation is consistent with previous experiments and numerical simulations about silicate dust aggregates. We estimate that the monomer radius of comet 67P has to be about 3.3–220 μm to reproduce its tensile strength using our model.

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1. Introduction

Planetesimal formation is one of the most important and unsolved issues of planet formation theory. In protoplanetary disks, submicrometer-sized dust grains are believed to coagulate, settle to the disk midplane as they grow, and form kilometer-sized planetesimals. There are several scenarios for planetesimal formation, such as gravitational instability (e.g., Goldreich & Ward 1973), streaming instability (e.g., Youdin & Goodman 2005; Johansen et al. 2007, 2011), and direct coagulation. In the direct coagulation scenario, dust grains grow larger by pairwise collisions. Recently, it has been proposed that dust grains become not compact but porous by pairwise collisions, and the properties of these fluffy dust aggregates have been investigated theoretically and experimentally (e.g., Kozasa et al. 1992; Ossenkopf 1993; Dominik & Tielens 1997; Blum & Wurm 2000; Wada et al. 2007, 2008; Suyama et al. 2008). The submicrometer-sized constituent grains are called monomers. Finally, it is found that planetesimals form via direct coagulation (e.g., Okuzumi et al. 2012; Kataoka et al. 2013a).

In recent years, the physical properties of comets have been investigated by observation and exploration. Comets are the most primitive bodies in our solar system and are thought to be leftover planetesimals. In 2014, Rosetta reached comet 67P/Churyumov–Gerasimenko (hereafter 67P). This mission pioneered orbiting and landing on a comet. 67P has many unexpected results (e.g., Fulle et al. 2016), and it is especially remarkable that its tensile strength was estimated. The tensile strength of the surface of 67P is 3–150 Pa (Groussin et al. 2015; Basilevsky et al. 2016), while that for the bulk comet is 10–200 Pa (Hirabayashi et al. 2016). This tensile strength depends on the composition and formation process of comets, i.e., planetesimals.

There are several experimental studies about the tensile strength of dust aggregates. Blum & Schräpler (2004) directly measured the tensile strength of dust aggregates whose volume filling factors are 0.2 and 0.54. They used dust aggregates consisting of monodisperse silica (SiO2) spheres with a 0.76 μm radius. In their experiments, a millimeter-sized dust aggregate was attached to two plates at its top and bottom, and then the two plates were pulled apart. Blum et al. (2006) conducted the same experiments using dust aggregates with volume filling factors of 0.23, 0.41, and 0.66. In addition to the monodisperse spherical silica monomers, they used irregularly shaped diamond monomers with a narrow size distribution and irregular silica monomers with a wide size distribution. Meisner et al. (2012) used dust aggregates consisting of quartz (crystallized SiO2) monomers with a size range from 0.1 to 10 μm and measured the tensile strength using the Brazilian disk test (e.g., Li & Wong 2013). Gundlach et al. (2018) also performed the Brazilian disk test to measure the tensile strength of dust aggregates composed of polydisperse spherical ice (H2O) monomers and monodisperse spherical silica monomers. They used silica monomers whose radii are 0.15, 0.50, and 0.75 μm to investigate the monomer radius dependence. Moreover, they succeeded in measuring the tensile strength of ice dust aggregates whose monomer radius is 2.4 μm on average.

On the other hand, there is only one numerical study about the tensile strength of dust aggregates. Seizinger et al. (2013) performed three-dimensional simulations to reproduce the experimental results by Blum & Schräpler (2004) and Blum et al. (2006). They used dust aggregates whose volume filling factor ranges from 0.15 to 0.6 and monomers are silicate spheres with 0.6 μm radius. In their simulations, a micrometer-sized cubic aggregate was attached to two plates, which is the same as previous experiments except for the size of dust aggregates; a millimeter-sized dust aggregate was used in the previous experiments. The interaction between two monomers is mainly based on Dominik & Tielens (1997). In addition, they introduced the rolling and sliding modifiers to make numerical simulations correspond with experimental results (Seizinger et al. 2012). To avoid monomers being peeled off the plate, they also used an artificial adhesion force as a "gluing effect." Although their results correspond well with the laboratory result, the influence of their artificial adhesion force and small aggregates should also be checked. They also obtained a fitting formula for the tensile strength as a function of the filling factor of dust aggregates. However, their formula does not include the dependence on the monomer size and material.

In this work, we numerically investigate the tensile strength of dust aggregates composed of single-sized spherical monomers. In previous works, a dust aggregate was attached to two plates, and then they were pulled apart (Blum & Schräpler 2004; Blum et al. 2006; Seizinger et al. 2013). The size of the used dust aggregates ranges from micrometers to millimeters, while planetesimals are kilometer-sized. To unravel the planetesimal formation mechanism, it is important to investigate the tensile strength of dust aggregates that are larger than kilometers. Therefore, we use the periodic boundary condition to remove the effects of plates. Moreover, we perform simulations using dust aggregates whose volume filling factors are lower than those of the previous works. Then, we find a power-law relation between the tensile strength and initial volume filling factor of dust aggregates whose filling factors range from 10−2 to 0.5. We will also construct a theoretical model to explain the power-law dependence. This model reproduces the dependence on all material parameters in our simulations.

This paper is organized as follows. In Section 2, we describe the settings of our simulations, which include the model of monomer interactions, initial dust aggregates, the periodic boundary condition, how to measure the tensile strength without plates, and an overview of our simulations. Then, we summarize our results of fiducial runs and the investigation of parameter dependence in Section 3. There are three numerical parameters: the number of monomers, boundary velocity, and the strength of the damping force. There are four physical parameters: the initial volume filling factor, monomer radius, surface energy, and the critical rolling displacement. We also find an analytical expression of the tensile strength of dust aggregates, compare our results with previous experiments (Blum & Schräpler 2004; Blum et al. 2006; Gundlach et al. 2018) and numerical simulations (Seizinger et al. 2013), and apply the analytical expression 67P in Section 4. Finally, we provide conclusions and discuss future works in Section 5.

2. Simulation Settings

We perform three-dimensional numerical simulations to measure the tensile strength of dust aggregates consisting of spherical monomers. In this section, we describe the settings of our simulations. First, we introduce the monomer interaction model based on Dominik & Tielens (1997) and Wada et al. (2007) in Section 2.1. In Section 2.2, we explain the damping force in the normal direction. The initial conditions of our simulations are statically and isotropically compressed dust aggregates investigated by Kataoka et al. (2013b), which is described in Section 2.3. At the boundaries of the calculation box, we set moving periodic boundaries in the x-axis direction and fixed periodic boundaries in the y- and z-axis directions, which is explained in Section 2.4. Thus, we can simulate one-direction stretching of dust aggregates. The details of the calculation method of tensile stress, which is the same as molecular dynamics, are summarized in Section 2.5. In Section 2.6, we describe an overview of our simulations.

2.1. Monomer Interaction Model

We calculate interactions of each connection between two monomers using the theoretical model by Dominik & Tielens (1997) and Wada et al. (2007). Based on the JKR theory (Johnson et al. 1971) and the following studies by Dominik & Tielens (1995, 1996), Dominik & Tielens (1997) carried out two-dimensional simulations of monomer interactions. To expand into three-dimensional simulations, Wada et al. (2007) tested their recipe, and then Wada et al. (2008) conducted three-dimensional simulations of dust aggregate collisions. In the model, there are four kinds of interactions: normal (sticking and breaking), sliding, rolling, and twisting. The material parameters needed to describe the interactions are the monomer radius r0, material density ρ0, surface energy γ, Poisson's ratio ν, Young's modulus E, and the critical rolling displacement ξcrit. These parameters of ice and silicate are listed in Table 1. To compare our results with those by Seizinger et al. (2013), we set the same values for silicate.

Table 1.  Material Parameters of Ice (Israelachvili 1992; Dominik & Tielens 1997)

Material Ice Silicate
Monomer Radius r0 (μm) 0.1 0.6
Material Density ρ0 (g cm−3) 1.0 2.65
Surface Energy γ (mJ m−2) 100 20
Poisson's Ratio ν 0.25 0.17
Young's Modulus E (GPa) 7 54
Critical Rolling Displacement ξcrit (Å) 8 20

Note. The parameters of silicate are selected according to Seizinger et al. (2013).

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If a rolling displacement exceeds the critical one, ξcrit, a monomer begins to roll inelastically. The critical rolling displacement has different values between the theoretical one (ξcrit = 2 Å, Dominik & Tielens 1997) and the experimental one (ξcrit = 32 Å, Heim et al. 1999). We adopt ξcrit = 8 Å as a fiducial value and investigate the dependence of our results on ξcrit in Section 3.3.

The rolling energy Eroll needed to rotate a monomer around its connection point by 90° is described as

Equation (1)

where R is the reduced monomer radius (Wada et al. 2007). The reduced radius R of monomer radii r1 and r2 is defined as

Equation (2)

Here, the reduced monomer radius is R = r0/2 because we assume no size distribution of monomers.

In our simulations, the maximum force needed to separate two sticking monomers (breaking) is

Equation (3)

2.2. Damping Force in Normal Direction

The force in the normal direction induces oscillation at each connection between two monomers. In reality, the oscillation would attenuate because of viscoelasticity or hysteresis of monomers (Greenwood & Johnson 2006; Tanaka et al. 2012). Therefore, we add an artificial damping force in the normal direction (Paszun & Dominik 2008; Suyama et al. 2008; Seizinger et al. 2012; Kataoka et al. 2013b). The dependence of our results on the damping force is investigated in Section 3.2.

We describe the damping force as follows. In the case in which two contacting monomers have their position vectors ${{\boldsymbol{x}}}_{1}$ and ${{\boldsymbol{x}}}_{2}$, and velocities ${{\boldsymbol{v}}}_{1}$ and ${{\boldsymbol{v}}}_{2}$, respectively, the contact unit vector ${{\boldsymbol{n}}}_{{\rm{c}}}$ is defined as

Equation (4)

(Wada et al. 2007). The damping force applied to each monomer is introduced as

Equation (5)

where kn is the damping coefficient, m0 is the monomer mass, tc is the characteristic time, and ${{\boldsymbol{v}}}_{{\rm{r}}}$ is the relative velocity (Kataoka et al. 2013b). When we calculate the damping force experienced by the monomer (${{\boldsymbol{x}}}_{1},{{\boldsymbol{v}}}_{1}$), ${{\boldsymbol{v}}}_{{\rm{r}}}={{\boldsymbol{v}}}_{2}-{{\boldsymbol{v}}}_{1}$ is the relative velocity of the other monomer (${{\boldsymbol{x}}}_{2},{{\boldsymbol{v}}}_{2}$). We adopt kn = 0.01 as a fiducial value.

The characteristic time is given by Wada et al. (2007) as

Equation (6)

where E* is the reduced Young's modulus of monomers 1 and 2 defined as

Equation (7)

In our simulation, the Young's modulus E1 = E2 = E and the Poisson's ratio ν1 = ν2 = ν are uniform.

2.3. Initial Dust Aggregates

The initial dust aggregates are statically and isotropically compressed ballistic cluster–cluster aggregations (BCCAs) investigated by Kataoka et al. (2013b). We set these initial conditions to simulate the planetesimal formation mechanism. The calculation boundary is treated periodically, thus we do not have to consider the aggregate radius.

2.4. One-direction Stretching by Moving Boundaries

We set moving boundaries in the x-axis direction and fixed boundaries in the y- and z-axis directions to measure the tensile strength of dust aggregates. The initial calculation box is a cube whose length on each side is L0. The length in the y- and z-axis directions does not change, while the length in the x-axis direction Lx increases. Therefore, the coordinates in the x-, y-, and z-axis directions are $-{L}_{x}/2\lt x\lt {L}_{x}/2$, $-{L}_{0}/2\lt y\lt {L}_{0}/2$, and $-{L}_{0}/2\lt z\lt {L}_{0}/2$, respectively.

The velocity at the boundary in the x-axis direction ${v}_{{\rm{b}}}\gt 0$ has to be constant and less than the effective sound speed of dust aggregates for static stretching. We investigate the dependence on the velocity in Section 3.2. The effective sound speed of dust aggregates ${c}_{{\rm{s}},\mathrm{eff}}$ is described as

Equation (8)

where P and ρ are the pressure and mean internal density of dust aggregates, respectively. Because the initial dust aggregates are statically and isotropically compressed, their pressure is given as

Equation (9)

(Kataoka et al. 2013b). From Equations (8) and (9), we can obtain the effective sound speed of dust aggregates as

Equation (10)

where ϕ = ρ/ρ0 is the volume filling factor of dust aggregates. Since vb is independent of time t, the length in the x-axis direction Lx can be written as

Equation (11)

We treat the coordinates and velocity of a monomer across a periodic boundary as follows. When a monomer passes the moving periodic boundary at x = Lx/2, its position x and velocity vx are converted as

Equation (12)

Equation (13)

On the other hand, in the case of the moving periodic boundary at x = −Lx /2, its position and velocity are converted as

Equation (14)

Equation (15)

At y = ±L0/2 and z = ±L0/2, the coordinates of a monomer are converted similarly, but its velocity is not changed.

2.5. Tensile Stress Measurement

We calculate tensile stress in the same way as Kataoka et al. (2013b) because we have no walls. This is different from Seizinger et al. (2013), who measured the tensile stress considering the force exerted on walls.

The tensile stress is calculated only in the x-axis direction as follows. At first, we assume a virtual box, which is the same as the calculation box. The equation of motion of the monomer i in the x-axis direction is described as

Equation (16)

where Wx,i is the force exerted from the walls of the virtual box on the monomer i and Fx,i is the total force from other monomers on the monomer i. We multiply Equation (16) by xi and take a long-time average with the time interval τ. The left side of Equation (16) becomes

Equation (17)

The first term on the right side of Equation (17) becomes zero when $\tau \to \infty $. Here, we define the long-time average as $\langle {\rangle }_{t}$ and take a summation of all monomers of Equation (16). Then, Equation (16) can be written as

Equation (18)

The left side of Equation (18) can be defined as

Equation (19)

which is the time-averaged kinematic energy in the x-axis direction of all monomers. The first energy term on the right side of Equation (18) is related to the tensile stress in the x-axis direction Px. Since the virtual box is the same as the calculation box, we obtain

Equation (20)

where $V={L}_{x}{L}_{0}^{2}$ is the volume of the calculation box. Therefore, Equation (18) gives an expression of the tensile stress Px as

Equation (21)

The total force from other monomers on the monomer i can be described as

Equation (22)

where fx,i,j is the force from the monomer j on the monomer i in the x-axis direction. Thus, Equation (21) can be written as

Equation (23)

because of the relation that fx,i,j = −fx,j,i. Equation (23) is different from that of Kataoka et al. (2013b) because we consider the tensile stress only in the x-axis direction.

We take an average of the tensile stress Px for every 10,000 time steps, at least. In some simulations, the tensile stress fluctuates, thus we take a longer time average to smooth it (see Section 3.1 for details). One time step in our simulation is $0.7{t}_{{\rm{c}}}=1.9\times {10}^{-11}$ s, and therefore 10,000 time steps corresponds to $1.9\times {10}^{-7}$ s.

2.6. Overview of Our Simulations

The overview of our numerical simulations is as follows. First, we randomly create a BCCA to change the initial condition. Next, we compress it statically and isotropically (Kataoka et al. 2013b). The compression of a BCCA corresponds to the formation of a planetesimal. It is necessary for the BCCA to be attached to all boundaries so that we can stretch it. Then, we stop compression and define this volume filling factor as the initial one ϕinit. Finally, we stretch it statically and one-dimensionally. Figure 1 shows the overview of our simulations.

Figure 1.

Figure 1. Overview of our simulations. Each picture shows a BCCA (left), a compressed aggregate (center), and a stretched aggregate (right). Each aggregate contains 16,384 ice monomers whose radius is 0.1 μm. In the center and right panels, the box with white lines shows the calculation box with periodic boundaries.

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3. Results

We perform 10 simulations with different initial dust aggregates for every parameter set. First, we perform fiducial runs to investigate what occurs in our stretching simulations in Section 3.1. Then, we show that the results do not depend on any numerical parameters, such as the number of particles N, boundary velocity vb, and the damping coefficient kn in Section 3.2. Finally, in Section 3.3, we investigate the dependence on physical parameters: the initial volume filling factor ϕinit, monomer radius r0, surface energy γ, and the critical rolling displacement ξcrit.

3.1. Fiducial Run

We measure the tensile stress of 10 runs for the fiducial parameter set. The fiducial values are N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. Figure 2 shows three snapshots of a fiducial run. Each particle represents a 0.1 μm radius ice monomer. The light gray monomers are in the calculation box with periodic boundaries, while the dark gray monomers are in the neighbor boxes. The box with white lines shows the final state of the calculation box. By stretching the dust aggregate, the chain-like structure appears.

Figure 2.

Figure 2. Snapshots of a fiducial run when N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. The calculation times are $t=0\,{\rm{s}}$ (top), $t=2.49\times {10}^{5}{t}_{\mathrm{step}}\sim 4.7\times {10}^{-6}\,{\rm{s}}$ (center), and $t=4.98\times {10}^{5}{t}_{\mathrm{step}}\sim 9.5\times {10}^{-6}\,{\rm{s}}$ (bottom), where ${t}_{\mathrm{step}}=0.7{t}_{{\rm{c}}}=1.9\times {10}^{-11}\,{\rm{s}}$ represents one time step. Each particle represents a 0.1 μm radius ice monomer. The light gray monomers are in the calculation box with periodic boundaries, while the dark gray monomers are in the neighbor boxes. The box with white lines shows the final state of the calculation box. We omit the boxes in front, behind, above, and below the calculation box for simplicity.

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Figure 3 shows the time evolution of tensile stress of 10 fiducial runs averaged for every 10,000 time steps (left) and 200,000 time steps (right). The volume filling factor at each time step is calculated as

Equation (24)

and the tensile stress is calculated according to Equation (23). We choose the number of time steps when the rate of change of the volume filling factor does not exceed 10%. As tensile displacement increases, the volume filling factor ϕ decreases and the tensile stress Px increases. The maximum value of tensile stress is called the tensile strength. To calculate the tensile strength for every parameter set, we find 10 maximum values of the obtained tensile stress and take an average of them.

Figure 3.

Figure 3. Tensile stress Px of 10 fiducial runs averaged for every 10,000 time steps (left) and 200,000 time steps (right) when N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. The yellow dashed lines show the compressive strength (Equation (9)) investigated by Kataoka et al. (2013b).

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3.2. Numerical Parameter Dependence

To investigate the dependence on the number of particles N, we plot tensile stress when N = 210 = 1024, N = 212 = 4096, N = 214 = 16384, and N = 216 = 65536 in Figure 4(a). Changing N corresponds to changing the size of the calculation box. Obviously, the tensile strength has no dependence on N. Because of the smoothness of the tensile stress plot and calculation costs, we set N = 16384 as the fiducial value.

Figure 4.

Figure 4. Tensile stress Px with different numbers of particles N (left), different boundary velocities vb (center), and different damping coefficients kn (right). The fiducial values are N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å.

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Figure 4(b) shows tensile stress when boundary velocity vb = 1, 10, and 100 cm s−1. All boundary velocities are less than the effective sound speed of dust aggregates cs,eff (Equation (10)). There is no difference among the three boundary velocities. Therefore, we can conclude that dust aggregates are stretched statically. We set vb = 10 cm s−1 as the fiducial value considering sampling rates of tensile stress and calculation costs.

Tensile stress with various damping coefficients is plotted in Figure 4(c). No damping force corresponds to kn = 0. We change the strength of damping force from weak damping (kn = 0.01) to strong damping (kn = 1). Undoubtedly, there is no dependence on the damping force in this range. We use kn = 0.01 for all the other simulations.

3.3. Physical Parameter Dependence

We measure the tensile strength of dust aggregates that have various initial volume filling factors as shown in Figure 5. The calculated tensile strength is proportional to ${\phi }_{\mathrm{init}}^{1.8}$ from the fitting. The tensile strength Px,max can be described with the initial volume filling factor ϕinit as

Equation (25)

where ${P}_{0}\sim 6\times {10}^{5}\,\mathrm{Pa}$ in this case. The analytical interpretation of Equation (25) is discussed in Section 4.1.

Figure 5.

Figure 5. Tensile strength Px,max as a function of initial volume filling factor ϕinit when N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. The blue and yellow dashed lines show the best fit for the tensile strength (Equation (25)) and the compressive strength (Equation (9)), respectively. The error bar corresponds to the standard deviation of 10 runs.

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To investigate the dependence of tensile strength on the monomer radius, we perform simulations in the case of ice monomers whose radii are 0.3 and 0.9 μm. Figure 6 shows the summary of the monomer radius dependence. The plotted dashed lines are based on Equation (31), which is an analytical expression of tensile strength (see Section 4.1). It is confirmed that the tensile strength is in inverse proportion to the monomer radius.

Figure 6.

Figure 6. Tensile strength Px,max as a function of initial volume filling factor ϕinit when N = 16384, kn = 0.01, γ = 100 mJ m−2, and ξcrit = 8 Å. The monomer radii are r0 = 0.1 μm (blue), ${r}_{0}=0.3\,\mu {\rm{m}}$ (orange), and ${r}_{0}=0.9\,\mu {\rm{m}}$ (green). The error bar corresponds to the standard deviation of 10 runs. The dashed lines represent Equation (31).

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To clarify the surface energy dependence, we calculate the tensile strength when γ = 50 and 25 mJ m−2 and plot it in Figure 7. The other parameters are the same as the fiducial values. The dashed lines represent Equation (31) (see Section 4.1). Obviously, the tensile strength is in proportion to the surface energy.

Figure 7.

Figure 7. Tensile strength Px,max as a function of initial volume filling factor ϕinit when N = 16384, kn = 0.01, r0 = 0.1 μm, and ξcrit = 8 Å. The values of surface energy are γ = 100 mJ m−2 (blue), γ = 50 mJ m−2 (orange), and $\gamma =25\,\mathrm{mJ}\,{{\rm{m}}}^{-2}$ (green). The error bar corresponds to the standard deviation of 10 runs. The dashed lines represent Equation (31).

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Finally, we investigate the dependence of tensile stress on the critical rolling displacement ξcrit in Figure 8. The critical rolling displacement is changed from ${\xi }_{\mathrm{crit}}=2\mathring{\rm A} $ (e.g., Dominik & Tielens 1997) to ${\xi }_{\mathrm{crit}}=32\mathring{\rm A} $ (e.g., Heim et al. 1999). Tensile stress has a marginal dependence on ξcrit because the main mechanism of displacement is rolling (see Section 4.1). On the other hand, tensile strength, which is the maximum value of tensile stress, has no difference. We can conclude that the tensile strength is almost the same even if the critical rolling displacement has uncertainty. Therefore, we fix ${\xi }_{\mathrm{crit}}=8\mathring{\rm A} $ in our simulations.

Figure 8.

Figure 8. Tensile stress Px with different critical rolling displacements ξcrit when N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, and γ = 100 mJ m−2. The critical rolling displacements are ξcrit = 2 Å (blue), ${\xi }_{\mathrm{crit}}=4\,\mathring{\rm A} $ (orange), ξcrit = 8 Å (green), ${\xi }_{\mathrm{crit}}=16\,\mathring{\rm A} $ (magenta), and ξcrit = 32 Å (brown).

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4. Discussions

Now, we discuss the obtained physical parameter dependence of the tensile strength of dust aggregates (Section 3.3) and apply our results to previous studies of experiments, numerical simulations, and comet 67P. In Section 4.1, we find an analytical expression of the tensile strength using material parameters: the initial volume filling factor, monomer radius, and the surface energy. Then, we compare our results with previous experiments and numerical simulations about silicate dust aggregates (Blum & Schräpler 2004; Blum et al. 2006; Seizinger et al. 2013; Gundlach et al. 2018) in Section 4.2. Finally, we apply our interpretation to comet 67P in Section 4.3.

4.1. Semi-analytical Model of Tensile Strength

The relationship between Px,max and ϕinit can be derived by considering the maximum force needed to separate two sticking monomers Fc and the radius of a dust aggregate ragg. When the tensile stress has a maximum value, the force Fc is applied on a connection between two monomers of a dust aggregate. This means that

Equation (26)

The radius of a dust aggregate is given as

Equation (27)

where D and Nagg are the fractal dimension and the number of monomers of a dust aggregate, respectively. The initial volume filling factor is described as

Equation (28)

and then the radius of a dust aggregate is obtained as

Equation (29)

From Equation (26), the tensile strength can be written as

Equation (30)

where C is a constant. The fractal dimension D of BCCAs is ∼1.9 (Mukai et al. 1992; Okuzumi et al. 2009).

Using the fitting result of Equations (3) and (25), we obtain

Equation (31)

In the case of an ice monomer with a radius of 0.1 μm, we find C = 0.12 ± 0.01.

We confirm Equation (31) from the perspective of energy dissipation. All energy dissipations, which are caused by the normal, sliding, rolling, twisting, and damping force in the normal direction, are plotted in Figure 9. The curves in Figure 9 run time-wise from right to left and arise during the stretching of a dust aggregate. The main energy dissipation mechanism is the rolling, which corresponds to the ξcrit-dependence of tensile stress (Section 3.3). The energy dissipation by the normal arises when the tensile stress has a maximum value. This energy dissipation is caused by connection breaking between two contacting monomers. For this reason, tensile strength is determined by the connection breaking, i.e., Fc.

Figure 9.

Figure 9. Energy dissipations of a fiducial run when N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. The energy dissipation mechanisms are the normal (orange), sliding (green), rolling (magenta), twisting (brown), damping (purple), and the total of all energy dissipations (blue). The vertical gray line represents the volume filling factor when tensile stress has a maximum value.

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To confirm that D ∼ 1.9 on a small scale of a dust aggregate in our simulations, we calculate the number of monomers inside the radius rin for five snapshots of a fiducial run and plot it in Figure 10. We take the snapshots during the continuous strain of the dust aggregate. The parameters of the fiducial run are N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. The method to count the number of monomers N(r < rin) is as follows. At first, we set a monomer in the calculation box as the center and count N(r < rin) including monomers outside the periodic boundaries. Next, we take an average of N(r < rin) for all monomers in the calculation box.

Figure 10.

Figure 10. Number of monomers inside the radius rin as a function of ${r}_{\mathrm{in}}/{r}_{0}$ when N = 16384, ${v}_{{\rm{b}}}=10\,\mathrm{cm}\,{{\rm{s}}}^{-1}$, kn = 0.01, ϕinit = 0.1, r0 = 0.1 μm, γ = 100 mJ m−2, and ξcrit = 8 Å. Five snapshots are represented by blue ($\phi ={\phi }_{\mathrm{init}}=0.1$), orange ($\phi =0.08$), green ($\phi =0.06$), magenta ($\phi =0.05$), and brown ($\phi =0.04$) lines. The blue and red dashed lines show the relationship when D = 2 and D = 3, respectively.

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Also, we plot N(r < rin) as a function of ${r}_{\mathrm{in}}/{r}_{0}$ when D = 2 and D = 3 in Figure 10. This relationship is derived by Equation (27) as

Equation (32)

On a small scale that $N(r\lt {r}_{\mathrm{in}})\lesssim 20$, all snapshot results mostly correspond to the relationship when D = 2. When the scale becomes large enough, dust aggregates have a fractal dimension of three.

4.2. Comparison with Previous Studies

To compare our results with previous experiments and numerical simulations, we perform simulations with the parameters of silicate listed in Table 1 and summarize the results in Figure 11. Both results by experiments (Blum & Schräpler 2004; Blum et al. 2006; Gundlach et al. 2018) and simulations (this work; Seizinger et al. 2013) correspond very well. This means that there is little influence from the artificial adhesion force introduced by Seizinger et al. (2013) and small aggregates whose sizes range from micrometers to millimeters. The right panel of Figure 11 is derived by Equation (31), i.e., ${P}_{x,\max }\propto {r}_{0}^{-1}$.

Figure 11.

Figure 11. Tensile strength Px,max of silicate dust aggregates of this work and previous studies, which contain various initial volume filling factors ϕinit and monomer radii r0 (left), and that scaled to a monomer radius of 0.6 μm (right). The filled circles show our simulation results when N = 16384 and kn = 0.01. Other material parameters of silicate are listed in Table 1. The error bar corresponds to the standard deviation of 10 runs. The dashed lines represent Equation (31), while the dotted line represents Equation (2) of Seizinger et al. (2013). The experimental results are denoted by open squares (Blum & Schräpler 2004), open circles (Blum et al. 2006), and open triangles (Gundlach et al. 2018). The monomer radii are 0.15 μm (magenta), 0.5 μm (green), 0.6 μm (blue), 0.75 μm (brown), and 0.76 μm (orange).

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Gundlach et al. (2018) measured the tensile strength of ice aggregates with the monomer radius of $2.38\pm 1.11\,\mu {\rm{m}}$, which is shown in Figure 12. We do not know which monomer radius determines the tensile strength of dust aggregates when the monomer radius has a size distribution. Therefore, we plot dashed lines derived with Equation (31) when r0 = 1.27 μm, ${r}_{0}=2.38\,\mu {\rm{m}}$, and ${r}_{0}=3.49\,\mu {\rm{m}}$. The experimental value is lower than the theoretical lines. From their low value of the tensile strength, Gundlach et al. (2018) inferred that the specific surface energy of ice, ${\gamma }_{\mathrm{ice}}$, has a value of $=0.02\,{\rm{J}}\,{{\rm{m}}}^{-2}$ at low temperatures ($\lesssim 150$ K). However, Gundlach & Blum (2015) also estimated ${\gamma }_{\mathrm{ice}}=0.19\,{\rm{J}}\,{{\rm{m}}}^{-2}$ from the constant sticking threshold velocity of $\sim 10\,{\rm{m}}\,{{\rm{s}}}^{-1}$ for $T\lt 210$ K in their ice impact experiments. The reason for low tensile strength in Gundlach et al. (2018) is thus unknown. We also confirm that the experimental value is higher than the compressive strength theoretically expected by Kataoka et al. (2013b) (Equation (9)).

Figure 12.

Figure 12. Tensile strength Px,max of ice dust aggregates of this work and the previous study. The dashed lines represent Equation (31). The experimental result when ${r}_{0}=2.38\pm 1.11\,\mu {\rm{m}}$ is denoted by the open triangle with error bars (Gundlach et al. 2018). The monomer radii are 1.27 μm (orange), 2.38 μm (blue), and 3.49 μm (green).

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4.3. Application to Comet 67P

We can estimate the monomer radius of comet 67P using Equation (31) as follows. From the exploration of 67P, it was found that the microporosity of 67P is 0.75–0.85 (Kofman et al. 2015), while the surface porosity is 0.87 (Fornasier et al. 2015). In other words, the volume filling factor of 67P is about 0.13–0.25. The averaged nucleus bulk density of 67P was estimated to be 0.533 ${\rm{g}}\,{\mathrm{cm}}^{-3}$ (Pätzold et al. 2016). In consideration of the high dust-to-water mass ratio of 67P (e.g., Fulle et al. 2016), its main material is not H2O ice, but silicate. Assuming that the bulk density is 0.533 ${\rm{g}}\,{\mathrm{cm}}^{-3}$ and the material density is 2.65 ${\rm{g}}\,{\mathrm{cm}}^{-3}$ (Table 1), we can estimate that the volume filling factor of 67P is about 0.20, which is consistent with the values of 0.13–0.25. Substituting ${P}_{x,\max }=3-200$ Pa (see Section 1), $\gamma =20\,\mathrm{mJ}\,{{\rm{m}}}^{-2}$, and ${\phi }_{\mathrm{init}}=0.20$ in Equation (33), we find that the monomer radius of 67P has to be 3.3–220 μm. To explain the low tensile strength of 67P using only our model, we have to consider a larger radius than that of interstellar materials.

Another idea to decrease the tensile strength is assuming an aggregate of aggregates (e.g., Blum et al. 2014, 2017) instead of a simple aggregate of monomers as discussed in this paper. The aggregate-of-aggregate model may explain the low strength with small monomers, but this is beyond the scope of this paper.

5. Conclusions

We investigated the tensile strength of porous dust aggregates whose initial volume filling factors ϕinit are from 10−2 to 0.5. We performed three-dimensional numerical simulations with periodic boundary condition to measure the tensile stress of dust aggregates. The monomer interaction model is based on Dominik & Tielens (1997) and Wada et al. (2007). The initial dust aggregates are statically and isotropically compressed BCCAs investigated by Kataoka et al. (2013b). At boundaries of the calculation box, we set moving periodic boundaries in the x-axis direction and fixed periodic boundaries in the y- and z-axis directions. The method used to calculate the tensile stress is the same as that used in the molecular dynamics. In our simulations, we created a BCCA at first, compressed it three-dimensionally, and then stretched it one-dimensionally. For every parameter set, we conducted 10 stretching simulations with different initial dust aggregates, found 10 maximum values of the obtained tensile stress, and took an average of them, which is called the tensile strength. Our main findings of the tensile strength of porous dust aggregates are as follows.

  • 1.  
    As a result of numerical simulations, we found that the tensile strength Px,max can be written as
    Equation (33)
    where Fc is the maximum force needed to separate two sticking monomers, ϕinit is the initial volume filling factor, r0 is the monomer radius, and γ is the surface energy.
  • 2.  
    We analytically confirmed the dependence in Equation (33). It is found that the tensile strength is determined by monomer connection breaking. This is consistent with the fact that Px,max is proportional to Fc, as shown in Equation (33).
  • 3.  
    It is confirmed that the energy dissipation during a stretching simulation supports the dependence in Equation (33). The energy dissipation caused by monomer connection breaking arises when the tensile stress has a maximum value. Also, the dependence on the initial volume filling factor corresponds to the fractal dimension of BCCAs, which is about 1.9 (Mukai et al. 1992; Okuzumi et al. 2009).
  • 4.  
    Equation (33) is consistent with the previous experimental (Blum & Schräpler 2004; Blum et al. 2006; Gundlach et al. 2018) and numerical (Seizinger et al. 2013) studies of silicate dust aggregates, while it is inconsistent with the previous experimental study of ice dust aggregates (Gundlach et al. 2018).
  • 5.  
    We estimated that the monomer radius of comet 67P has to be 3.3–220 μm using Equation (33). Assuming that the main material of 67P is silicate and its volume filling factor is about 0.20, we obtained the monomer radius to reproduce its tensile strength of 3–200 Pa.

From the point of view of planet formation, the conclusion that the monomer radius of 67P has to be 3.3–220 μm is inconsistent with the typical radius of dust monomers in the interstellar medium: submicrometer. To reduce the monomer radius of 67P, other mechanisms, such as sintering (e.g., Sirono & Ueno 2017), to decrease the tensile strength of dust aggregates, are needed.

We thank Satoshi Okuzumi for fruitful discussions.

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10.3847/1538-4357/ab09f7