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(Invited) Visualization of Charge Density Distribution in Parallel-Plate Dielectric Barrier Discharge Under Atmospheric-Pressure Air

© 2023 ECS - The Electrochemical Society
, , Citation Atsushi Komuro 2023 Meet. Abstr. MA2023-01 1502 DOI 10.1149/MA2023-01201502mtgabs

2151-2043/MA2023-01/20/1502

Abstract

Dielectric barrier discharge (DBD) is one of the atmospheric nonequilibrium plasma and is typically driven by sinusoidal or pulse voltage with electrodes that dielectric is inserted. DBD has been used in some industries such as plasma medicine and material processing. However, the fundamental process of DBD has not been elucidated yet. When a parallel plate DBD is driven by sinusoidal voltage under atmospheric pressure, numerous filamentary discharges called microdischarges (MDs) are observed. The surface charge deposited on the dielectric after the discharge plays a major role in the behavior of these MDs. As the MD develops during the gap and reaches the dielectric surface, a surface discharge occurs and deposits the charge on the dielectric surface.

We performed dielectric surface charge measurements using Bi4Ge3O12, a Pockels crystal, in a short-gap, parallel-plate DBD of 0.5 and 0.3 mm driven by a sinusoidal high voltage. The high-speed camera enabled measurement of the spatio-temporal distribution of surface charge and estimation of the net electric field and the characteristics of microdischarges (MDs).

The net electric field strength in the gap was estimated from the measurement results. The axial reduced electric field strength generated by the surface charge was found to be equivalent to 50-60% of the peak value of the applied electric field with all the voltage amplitude and gap length in this study, and the gap electric field after discharge was suppressed to less than 100 Td. Such a strong field keeps the MDs in a nonequilibrium plasma and also prevents re-discharge in the same position at the half cycle. On the other hand, the lateral electric field strength generated by the surface charge is largely characterized by the charge distribution—i.e., the voltage amplitude, gap length, and charge polarity—as mentioned above. Higher amplitude of applied voltage leads to an increase in the area of high lateral electric field strength above 100 Td. Compared to the gap length of 0.5 mm, the lateral electric field weakened, while the axial electric field generated by the surface charge was stronger in the gap length of 0.3 mm. As for the relationship between the charge polarity and the lateral electric field, the lateral field at the anodic dielectric, which the negative charge is deposited on, is dominant in the region of less than 100 Td. Meanwhile, on the cathodic dielectric, which the positive charge is deposited on, the area of above 100 Td is larger. That is, the strong lateral electric field can be observed near the cathodic dielectric, rather than the anodic dielectric. Thus, different chemical reactions may occur in the vicinity of the anodic and cathodic dielectrics, respectively, because of the difference in the drifting charged particles and the lateral field strength.

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10.1149/MA2023-01201502mtgabs