Abstract
We report 31P NMR studies of an oriented polycrystalline superconductor of Ba0.5Sr0.5Fe2(As1−xPx)2 with x ∼ 0.4 (Tc = 29 K) at T = 14−325 K and B0 = 1 and 5 T. The 31P Knight shift Kab at B0 ⊥ c shows a nearly T-independent uniform spin susceptibility above Tc and a spin singlet decrease below Tc. The 31P nuclear spin-lattice relaxation rate 1/T1 shows an asymptotic behavior of a + bT (a and b are constants) at T > 100 K and the minimum at 40 K with an upturn toward Tc. The a term in 1/T1 indicates the presence of two-dimensional antiferromagnetic spin fluctuations. The negative θ = −15 K of the Curie-Weiss-type antiferromagnetic spin susceptibility in the analysis of 1/T1T suggests antiferromagnetic instability in the superconducting state. Discussions are made from the self-consistent renormalization (SCR) theory for the spin fluctuations with interlayer correlation.
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