Abstract
Spectral components of continuous squeezed fields are entangled. In this article we review and clarify this phenomenon by analyzing systematically the relations between the correlations of modes filtered from stationary continuous fields and the cross-power spectrum between the operators of the corresponding spectral components. Moreover, we study the specific spectral components that are filtered in homodyne or heterodyne detections and their entanglement properties. In particular, we establish the equivalence between two-mode squeezing variance and logarithmic negativity for the spectral components of continuous stationary fields, thereby demonstrating that the measurement of the homodyne or heterodyne spectrum is, in fact, a direct measurement of the logarithmic negativity between specific spectral modes. As an illustrative example, we apply these concepts to the analysis of entanglement in ponderomotive squeezing.
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1. Introduction
Quantum optical fields are exploited in the development of a large class of new technologies which make use of quantum mechanics to push their efficiency to the limit [1]. In particular, squeezed light plays a pivotal role in the continuous-variable domain [2–5]. After the first experimental demonstrations of optical squeezing, both in the continuous-wave [6, 7] and in the pulsed regime [8], and of the corresponding Einstein–Podolsky–Rosen (EPR) entanglement [9–11], nowadays squeezed optical fields are routinely produced and employed in many experiments aimed at investigating the potentiality of quantum-based technologies. They range, for example, from the demonstration of quantum information tasks such as quantum teleportation [12, 13] and other essential elements of scalable universal quantum computation [14–18] to the design of high-resolution metrology applications [19–23], of novel spectroscopic methods [24, 25], and of enhanced optical communication schemes [26].
Squeezing and entanglement are two very related concepts. In practice squeezed fields are, for example, used to produce two-mode entangled resources by simply mixing them on beam splitters [10, 12, 16]. From a more theoretical point of view, squeezing variance can be used to construct entanglement criteria [27–30]. It is also well known that the spectral components of continuous-wave squeezed light are endowed with non-trivial correlations [31–35]. In particular, specific spectral modes of continuous squeezed fields are entangled [36–39], realizing EPR spectral beams that have been proposed as convenient quantum communication channels [37, 40].
In this article we study squeezed continuous fields in the stationary regime, and we analyze the entanglement properties of the corresponding spectral components. We aim at establishing a direct connection between the entanglement theory of continuous-variable systems and the spectral properties of squeezed light fields in the stationary continuous-wave regime. The spectral modes of a continuous field can be operatively defined as the temporal modes filtered from the total field, with a long time filter. Their entanglement and squeezing properties are therefore readily defined as the long time limit of those that are found for finite temporal modes. By employing this approach, we derive general conditions for entanglement and squeezing between two spectral components of stationary continuous fields, and we show that their two-mode squeezing variance can be expressed in terms of the corresponding logarithmic negativity. We also discuss the properties of the specific spectral modes that are probed with homodyne and heterodyne detection [41, 42], and we establish that the squeezing spectrum that can be measured with these techniques can be interpreted as a direct measurement of the logarithmic negativity between specific spectral modes.
Finally, we apply these ideas to the analysis of ponderomotive squeezing [43–46], namely the squeezing that is obtained as a result of the optomechanical interaction between a mechanical resonator and the light in an optical cavity. Optomechanics provides a novel approach to the area of quantum non-linear optics, which recently has attracted much attention for its potential applications in quantum-enhanced technologies [47, 48]. In this work, we investigate a two-sided cavity with a membrane in the middle, and we identify the spectral components of the output fields that exhibit larger entanglement and that are experimentally accessible with homodyne and heterodyne techniques.
Part of this article comprises a review of already known results, however, rephrased with the intent of providing a clear and complete introduction to the scope of our research. In particular, in our presentation, the revision of established concepts is instrumental to the identification and full understanding of the new results concerning the relationship between entanglement and squeezing in continuous stationary fields that constitute the central outcome of this article. In detail, the article is organized as follows. In section 2 we review the basic properties of continuous fields and of their spectral properties. We introduce the filtered temporal modes and study the correlations of the corresponding field operators in the stationary regime. In section 3 we demonstrate the equivalence between logarithmic negativity and two-mode squeezing variance of the spectral components of stationary continuous fields. In section 4 we review homodyne and heterodyne detection techniques and study how they can be used to directly measure the logarithmic negativity between spectral modes. Then, in section 5, we apply the concepts developed in the preceding sections to ponderomotive squeezing. Finally, in section 6, we draw our conclusions and discuss some possible outlooks. The three appendices provide additional information regarding, respectively, the basic properties of entanglement and squeezing of discrete bosonic modes, the homodyne and heterodyne techniques, and the input–output theory applied to the investigation of an optomechanical system.
2. Continuous quantum optical fields
In this section we introduce the objects of our investigation, namely continuous fields, and we discuss the properties of temporal modes that can be filtered from them [49–51]. In particular we define the operators for the spectral components in terms of the modes that are filtered with a long-time filter and that describe narrow bands of frequencies. These operators are particularly suited for the study of the entanglement properties of the spectral components of continuous fields using standard techniques of entanglement theory.
In detail, we investigate the freely propagating continuous field E(t) at the output of a quantum optical system. It can be decomposed into the positive and negative frequency components
, with
and
, where σ is the cross section of the propagating field and
is the annihilation operator for the spectral component at frequency ω that satisfy the standard commutation relation
. In general, in an optical system, only a relatively narrow band of frequencies
is relevant. This band is centered around the carrier frequency
of the signal field E(t), which is typically defined by the frequency of a laser driving the system and fulfills the relation
. In practice the relevant bandwidth is set by the typical line width Γ of the system under investigation and eventually by the response time, T, of the detector such that
. Under these conditions the range of frequency integration in the expression for the field can be extended from
to
and the relevant wave numbers k can be approximated with the central value
. By this means the quantum optical continuous field can be expressed as

where we have introduced the continuous field annihilation operator a(t). It is related to the operators for the spectral components by the Fourier transform
, where here ω is the frequency relative to the carrier. It is also useful to introduce the operators
relative to the carrier frequency, which are equal to the Fourier transform of a(t):

and
. These operators satisfy the standard commutation relation for continuous fields:

2.1. Filtered modes and spectral components of the field
In reality one has access only to a finite time interval (and correspondingly to a finite band of frequencies) of the total field a(t). These detectable intervals of the total field correspond to specific temporal modes. They can be physically defined, for example, by the temporal profile of the pumping field in pulsed experiments [8, 10, 52–54], they can also be extracted by post-processing the previously recorded time signal [55, 56], or they can be selected by the measurement apparatus as a result of the corresponding response and detection times [56–59]. In particular, in the case of experiments involving stationary fields, the detection time can be sufficiently long to select a well-defined spectral component of the total signal (as achieved, for example, with an electronic spectrum analyzer) [6, 7, 42].
In general a temporal filtered mode can be introduced in terms of a filter function
, which defines the time profile of the mode with a duration of order τ. Correspondingly, it defines a band of spectral components, of width
, that are combined into the filtered signal [60, 61]. The generic form for the operators of a filtered mode can be expressed as

with
, and where the symbol
indicates filtered quantities. The parameter Ω defines the central frequency of the filter, and the filter function
is real and normalized according to

Consequently, the filtered operators are discrete bosonic operators which satisfy the standard commutation relation

The corresponding equivalent form of the filtered operators, in terms of the spectral components of the field, is

where
is the Fourier transformed filter function
which peaks at
and has a width on the order of
.
Two particular cases are worth mentioning: the exponential filter with
and
, which has been used, for example, in [57] to introduce the physical spectrum of light; and the step-filter function

which we will connect to homodyne and heterodyne detection techniques in the following. In this form the time t in the filtered operator
corresponds to the final time of the filtering process, that is,
Although not strictly relevant to the results presented in this article, this choice is physically motivated by the fact that in this way we define, at time t, a causal operator
which depends only on the past of the continuous field a(t) [60].
In the limit of long filtering times,
, the filter selects a single spectral component of the field. In the following we will focus on the spectral components of stationary fields for which we will use the following simplified notation:

where we drop the label τ, the limit symbol, and the time argument t. In particular, the time t in these operators is irrelevant for stationary fields, in the sense that (as shown in the next section) the correlations of operators of this form, in the limit of large τ, are independent of the time arguments.
We finally note that we are describing the field in a reference frame rotating at the carrier frequency
; therefore
is, in fact, the operator for the spectral component of the field at the sideband frequency
2.2. Correlations of filtered spectral modes of stationary fields
In this article we are interested in the squeezing properties of the electromagnetic field, which refers to reduced fluctuations or reduced variance of specific quadratures below the vacuum noise level, and in the corresponding entanglement features. Squeezing can be revealed from the analysis of the second-order correlations of field operators. Therefore in this section we analyze the basic properties of the correlations of filtered modes. In particular we focus on the spectral properties of stationary fields. The corresponding field operators, a(t) and
, have diverging correlation functions as a consequence of the commutation relations in equation (3). In this case it is therefore instructive to analyze the fluctuations of the spectral modes in terms of the filtered spectral operators defined in equation (6), whose correlations, in contrast, are always finite also in the limit of long integration time
. This approach is particularly useful for the study of the corresponding entanglement properties, and it has the advantage of providing a clear physical definition of discrete modes corresponding to the specific spectral components, hence allowing for a transparent application of the techniques developed in entanglement theory, which indeed deals with discrete modes (see appendix
Let us study the correlations between the spectral components of two stationary continuous fields with annihilation operators
and
respectively, which fulfill the commutation relation
. (The same results that we discuss hereafter for two continuous fields can be applied with minor modifications to different spectral components belonging to a single field.) By straightforward application of the Wiener–Khintchine theorem, we find that all the information about the correlations between the spectral components is contained in the power spectrum matrix
, defined as the Fourier transform of the two-time stationary correlation matrix, which can be expressed in terms of the elements of the column vector of operators
as the matrix
, whose elements are
, where
are vector indices, not to be confused with the indices of the modes. To be specific,

where we use the fact that two-time correlation functions of stationary signals depend only on the difference of the time arguments. In particular the correlations between the Fourier-transformed operators
are diverging and are related to the power spectrum matrix by

To gain insight into the physical meaning of these diverging quantities we employ the narrow filtered modes introduced in the preceding section. We construct the vector of filtered spectral components
, which is given by
, and we compute the corresponding matrix of correlations:

These quantities can be evaluated by noting that for large τ, the square modulus of the filter function approaches a delta function,
, whereas its integral goes to zero,
. And, likewise, given a generic finite function
, the relation

holds. Consequently equations (10) and (12) can be used in equation (11) to find

which shows that the power spectrum is directly related to the correlations of narrow filtered modes. In other terms, in the limit of large integration time τ, i.e., when the bandwidth selected by the filter is sufficiently small, the correlation functions reduce to the power spectrum of the continuous field [57]. This result is valid when τ is much larger than the decay time of the signal correlations
(the memory time of the signals),
. We note in particular that this relation implies the stationarity of the signal, which is reached on a time scale on the order of
.
The correlations between two modes are conveniently analyzed in terms of the corresponding correlation matrix, from which the corresponding squeezing and entanglement properties can be readily derived (see appendix
is not a correlation matrix for two modes. In fact, it contains the correlations between the four spectral modes corresponding to the two pairs of sidebands at the frequency
of the two continuous fields. On the other hand, the elements of the power spectrum matrix can be used to construct the correlation matrix for two narrow modes filtered from the two stationary continuous fields as follows. We consider two modes, at frequencies Ω and
, respectively described by the filtered operators

where the narrow bandwidth limit
is implicit in their definition (see equation (8)). The corresponding correlation matrix is defined using the vector
, as
, and can be expressed in terms of the elements of the power spectrum matrix defined in equation (13) as

We finally note that
is equal to the power spectrum matrix
only at zero frequency,
.
3. Equivalence between two-mode squeezing variance and logarithmic negativity of the spectral components of stationary continuous fields
Having introduced our notation in the previous section, and having reviewed the basic properties of stationary continuous fields, we are now in a position to study the general conditions for squeezing and entanglement between two spectral components, which can be inferred from equation (15). In particular, in the case of Gaussian states, we establish the equivalence between the logarithmic negativity and the two-mode squeezing variance of two spectral modes.
In general, given two modes described by the operators a1 and a2, two-mode squeezing is characterized by non-vanishing correlations of the form
and
. According to equation (15), the correlation between the annihilation operators for two filtered spectral components of stationary fields,
and
, can be non-vanishing only for opposite frequencies, that is, when
. In this case the matrix in equation (15) reduces to the form

where

with
real and positive. Here we have used the general properties of the power spectrum matrix
, where
is the 2 × 2 identity matrix and the missing blocks are null matrices, and
, i.e.,
. Equation (16) represents the general form for the correlation matrix between two spectral components at opposite sideband frequencies of stationary continuous fields. This matrix can be exploited to derive general results regarding the corresponding squeezing and entanglement properties.
In general squeezing refers to the reduced fluctuations of field quadratures. Let us therefore define the quadrature operators for a spectral mode:

Thereby we can formalize the condition for two-mode squeezing of the two spectral components as follows. The two components are two-mode squeezed when the variance of a generic composite quadrature of the form

is below the shot noise level for some value of
(see appendix
is constant, the average of a corresponding filtered mode is given by
, and it approaches zero for large τ and for non-zero values of Ω. Therefore, according to our definitions, the fields are two-mode squeezed if for some values of
the autocorrelation function of the combined quadrature

is smaller than 1,
. More generally one can construct composite quadratures with different weights of the two components:

It has been shown [29] that the variance of quadratures of this form can be used to define entanglement criteria. Specifically, when the relation

is satisfied for some values of
and
, the two modes are entangled. In general this is a sufficient condition for entanglement, but it is also necessary in the case of Gaussian fields and for an appropriate choice of
. The calculation of the autocorrelation function of these composite quadratures is straightforward using the matrix of correlations in equation (16). The result is

In particular, we find that
; hence, in our case, the condition for entanglement reduces to
. The corresponding optimized squeezing spectrum can be defined as the minimum of this quantity over the quadrature of the field. Specifically we can identify two different minimization strategies. If we restrict the quadratures to composite quadratures that are a symmetric superposition of the two components (
) as in equation (19), the minimization runs only over the phases
, and the corresponding phase-optimized squeezing spectrum takes the general form

This is the quantity that is obtained, for example, by the homodyne measurement of a continuous field, where the phases
, in equation (22), are directly related to the phase of the local oscillator (see section 4 for further details). If, on the other hand, we consider the more general quadratures with the two components scaled by the factors
as in equation (20), the minimization can be performed both over the phases and over the parameters
, and the corresponding globally optimized squeezing spectrum reduces to

In general
, and they are equal in the case of symmetric spectral components, for which
. In the next section we describe how to measure both quantities in a few specific cases with homodyne and heterodyne techniques. Here we emphasize that the occurrence of
implies that the entanglement criterion in equation (21) is satisfied, and in turn, it means that a squeezing spectrum smaller than 1 is always a signature of entanglement. We further note that equation (23) is, indeed, smaller than 1 if and only if

Consequently this relation can be interpreted as a sufficient condition for the entanglement between the spectral components at opposite sideband frequencies of stationary continuous fields. And, as already noted, it is also a necessary condition in the case of Gaussian fields.
Let us now focus on the Gaussian regime. In this case the logarithmic negativity, which is a measure of bipartite entanglement [62], can be expressed as

where the parameter ν is equal to the smallest symplectic eigenvalues of the covariance matrix corresponding to the partially transposed state of the two modes (see appendix
is equal to the squeezing spectrum in equation (23),

This is a general result that is valid for the spectral components of stationary continuous fields. (A specific example has been discussed in [63].) In particular, this relation implies that, if the two stationary fields are Gaussian, then a measure of the minimum variance of a composite quadrature of two spectral components, of the form of equation ( 20 ), is a direct measurement of the corresponding logarithmic negativity.
4. Homodyne and heterodyne detection of the spectral components of stationary continuous fields
The quadratures of continuous electromagnetic fields are routinely measured in experiments with homodyne and heterodyne techniques [5, 41, 64–67]. The photocurrents resulting from homodyne and heterodyne detections are, in fact, proportional to specific quadratures of the detected field. In turn, the power spectrum of the photocurrent, namely the homodyne or heterodyne spectrum, measures the fluctuations of the quadratures at specific frequencies. Such spectra are therefore directly related to the squeezing and entanglement properties of the spectral components of the electromagnetic field, and in particular to the squeezing spectra defined in equations (22) and (23). Specifically, we will show that the autocorrelation function of the photocurrent minimized over experimentally accessible parameters such as the phase of the local oscillator can always be cast in the form of equation, (22) or (23), with corresponding parameters
and m evaluated for specific spectral modes. This justifies the interpretation of the optimized homodyne and heterodyne spectra as a direct measurement of the logarithmic negativity of these modes.
4.1. Single-mode homodyne spectrum and entangled spectral components
In homodyne detection the signal field is mixed on a 50:50 beam splitter with a strong monochromatic field (the local oscillator) at the same frequency as the carrier signal. The fields at the two output ports of the beam splitter are detected and the corresponding photocurrents are subtracted, resulting in a signal that contains information about a field quadrature [65] and that can be described by a photocurrent operator of the form (see appendix

where θ is the phase of the local oscillator. The power spectrum of the photocurrent contains information about the spectral components of the detected field, and in particular it quantifies the strength of the fluctuations at specific frequencies. We will refer to it as the homodyne spectrum, and it can be expressed as the autocorrelation function of the filtered photocurrent, integrated over a long time τ, of the form
. In detail, the homodyne spectrum can be written as

We note that, for stationary processes, this quantity is independent of the phase of the filter φ (see appendix
, one uses an exponential oscillating function, as in the filters of section 2.1, in place of the sinusoidal function introduced earlier. The use of a sinusoidal function is, however, more convenient because, in this case, the filtered photocurrent is a Hermitian operator, thereby making the relation between the photocurrent and the field observables more transparent. Specifically the filtered photocurrent in the limit of long filtering time can be expressed as the sum of two filtered quadrature operators for the two spectral modes at frequencies
(see appendix

Similar to equation (19), this is a symmetric superposition of two quadratures, defined as in equation (18), corresponding to the two spectral components, which in this case are filtered from the same field, and whose annihilation operators are

as illustrated in figure 1. The corresponding single-mode homodyne spectrum (where, single-mode, indicates that its results form the detection of a single continuous field) is equal to equation (22) with
and
, i.e.,
, where

Thus, the single-mode phase-optimized squeezing spectrum, which is experimentally accessible by tuning the phase of the local oscillator,
, is equal to equation (22) evaluated for the parameters in equation (31). When it is smaller than one, it indicates that the two sideband modes
are entangled [37–40]. Their logarithmic negativity, which as discussed in section 3, is directly related to the squeezing spectrum in equation (23), could be measurable if one could construct a filtered photocurrent similar to equation (20), which is a non-symmetric superposition of the quadratures of the two modes. This photocurrent is, in fact, achievable by combining two filtered photocurrents detected at appropriately tuned phases of the local oscillator θ and of the filter φ. Specifically one should first detect the filtered photocurrent
for some value of θ and φ and then a second one,
, with the phases tuned to different values
and
. The two photocurrents are then summed, resulting in the total photocurrent

which we have appropriately normalized, and where

We note that equation (32) has, indeed, the form of the composite quadrature defined in equation (20). The corresponding single-mode globally optimized squeezing spectrum
is then equal to equation (23) evaluated for the parameters in equation (31), and it can be measured by minimizing the homodyne spectrum over the phases of both the local oscillator and the filter. In particular, although the tuning the filter phases,
and
, can be, in principle, achieved by recording the photocurrent for a sufficiently long time and then post-processing the recorded signal, the phases of the local oscillator,
and θ', must be adjusted during repeated homodyne measurements.
Figure 1. Single-mode homodyne detection: a stationary continuous field is detected by homodyne techniques and the resulting filtered photocurrent is a superposition of spectral components at opposite sideband frequencies
.
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Standard image High-resolution image4.2. Two-mode homodyne spectrum and entangled spectral components
In the preceding section we saw that the single-mode homodyne spectrum, which is measurable from a single stationary continuous field, provides information about the entanglement between two spectral components. Let us now study the two-mode squeezing spectrum obtained from the combination of two homodyne photocurrents which result from the measurement of two signal fields
and
, as depicted in figure 2. This strategy detects the correlations between four spectral components [68]. Specifically, we consider the situation in which the photocurrents corresponding to the two detected fields,
and
, have the form of equation (27) and are combined to construct the total photocurrent

where we have introduced the scaling parameters
and
, which weight the two quadratures differently and hence provide a means to select arbitrary collective modes as discussed hereafter. These parameters are controllable experimentally, including the asymmetrical amplification and/or attenuation of the two photocurrents. The total photocurrent is then analyzed by frequency. As in the preceding case, the filtered photocurrent
can be decomposed into two spectral components at the frequencies
:

where
, and where we have introduced the quadrature operators for the collective spectral modes defined as

with the collective annihilation and creation operators given by

where
and
. Also in this case, the filtered photocurrent is a composite quadrature of the from of equation (29). Thus, although it is constructed from the collective operators in equation (37), we can still apply the results of section 3 to conclude that the two-mode squeezing spectrum,
, obtained as the minimum over the phases
of the autocorrelation function of the filtered current, has the form of equation (22) but is evaluated with the parameters

where

for
. We remark that
is found by minimizing the autocorrelation function of the photocurrent in equation (35) over
only, whereas
and
define the specific collective modes that are being probed and are fixed. Therefore, in this case the condition
indicates the entanglement of the collective modes described by the operators in equation (37), each of which is a superpositions of the spectral components at the same sideband frequencies of the two fields. Moreover, as with the discussions of the single-mode homodyne spectrum, the corresponding logarithmic negativity can be, in turn, measured by summing two filtered photocurrents, at different phases, of the form of equation (35) and then calculating the corresponding autocorrelation function. The two-mode squeezing spectrum
is then found by minimizing this quantity over the phases of both the local oscillator and the filter, and the result, in full similarity with the single-mode squeezing spectrum, is equal to equation (23) but now evaluated for the parameters in equation (38).
Figure 2. Two-mode homodyne detection: two stationary continuous fields are detected by homodyne techniques. The two photocurrents are summed and then analyzed by frequency. As in single-mode homodyne detection, the resulting total filtered photocurrent is a superposition of spectral modes at opposite sideband frequencies
. However, here each spectral mode [
] can be decomposed as the superposition of two spectral components [
and
] at the same sideband frequency, each filtered from one of the two fields.
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Standard image High-resolution image4.3. Detecting single spectral components with homodyne techniques
As discussed in the previous sections, it is possible to construct arbitrary superposition of spectral modes at opposite sideband frequencies by the superposition of two homodyne photocurrents. The corresponding total photocurrent is then given by equation (32). Similarly, when the phases in equation (33) are set to some values for which one of the two parameters
is equal to zero, then a single spectral mode is detected.
When applied to two distinct fields, this approach would permit the investigation of the correlations between two distinct spectral modes each belonging to a different field. Let us, for example, assume that we repeat the pair of measurements resulting in the total photocurrent in equation (32) for two different continuous fields
and
. The two resultant composite filtered photocurrents are then, in general, given by
with the parameters defined as in equation (33) and where here j = 1, 2 distinguishes the parameters corresponding to the measurements of the first and second fields respectively.
If, in each pair of measurements, we tune the phases of the local oscillators and of the filtersto certain values for which
and
so that
, then each composite photocurrent is proportional to a quadrature of a single spectral component corresponding respectively to the annihilation operators

The two photocurrents are then summed together, after being multiplied by appropriately chosen scaling factors
, so that the resulting total photocurrent is

where the single-mode quadratures
are defined in equation (18). Thus, this protocol detects the combined quadrature defined in equation (20). The corresponding squeezing spectrum,
, defined for
, as the minimum of the autocorrelation function of the total photocurrent over
and
, is equal to equation (22) and is obtained by appropriately tuning the phases of the local oscillator and the filter during repeated homodyne measurements. Similarly,
, defined as the minimum of the power spectrum of the total photocurrent over
,
and
, is equal to equation (23). In particular, also in this case we can conclude that this quantity is equivalent to the logarithmic negativity between
and
when the fields are Gaussian.
4.4. Two-mode heterodyne spectrum and entangled spectral components
An alternative strategy for probing single spectral modes and hence for measuring the squeezing spectrum, as well as the logarithmic negativity between two distinct spectral components of two distinct fields, as in section 4.3, is based on heterodyne measurements.
In heterodyne techniques, the local oscillator is detuned from the carrier frequency of the signal field by a quantity
, and the corresponding operator for the photocurrent reads

Hence, the corresponding filtered photocurrent,
, is the superposition of the quadratures for the spectral components at the frequencies
, namely
. Thus, whereas homodyne detection probes spectral components at opposite sideband frequencies, heterodyne techniques measure two components asymmetrically located with respect to the carrier frequency of the signal field but symmetric with respect to the local oscillator frequency, which, in our description (where all frequencies are relative to the carrier signal), is equal to Δ (see figure 3).
Figure 3. Single-mode heterodyne detection: a stationary continuous field is detected by heterodyne techniques with the local oscillator at the frequency Δ relative to the carrier frequency of the signal. The detected photocurrent is spectrally analyzed at the frequency
. The resulting filtered photocurrent is a superposition of spectral components at the frequencies Ω and
.
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Standard image High-resolution imageIn particular heterodyne techniques can be used to detect a single spectral component, as discussed in the following. Say we want to detect the component at frequency Ω; then we set the detuning Δ at a value much larger than the typical bandwidth of the signal
, which is the band of frequencies that are populated by the signal photons. We also assume that the frequency Ω is a relevant frequency for the field
. Then the corresponding heterodyne photocurrent is filtered at the frequency
so that, as depicted in figure 3,
is the superposition of the field quadratures at the frequencies Ω and
:

Since the signal covers a bandwidth much smaller than Δ, the mode at
is basically in a vacuum and only the photons of the sideband Ω are detected. However, in doing this the vacuum fluctuations of the empty component at
are added to the signal, resulting in higher noise.
This approach can be exploited to measure the correlations between two spectral modes belonging to two separate fields. Specifically the two-mode heterodyne spectrum is obtained when detecting two signals with two heterodyne measurements (with
). The corresponding photocurrents are filtered independently at the frequencies
and
respectively, and then combined, with appropriately chosen scaling factors
, to construct the total filtered photocurrent
. If, in particular, we are interested in the spectral components at frequency Ω of the first field and at frequency
of the second such that
, we consider the filtered photocurrents at the frequencies
and
. As in equation (41) they are equal, respectively, to the superpositions of the two quadratures at frequencies Ω and
of the first field and of the two quadratures at frequencies
and
of the second. Correspondingly, the total photocurrent is given by

where the quadrature operators for a single component are defined in equation (18). Its autocorrelation function is therefore given by

where the term
on the right is due to the vacuum fluctuations of the spectral modes at
, the collective quadrature
has the same form of the one defined in equation (20), and its autocorrelation function, which is given in equation (22), quantifies the correlations between the modes
and
.
Also in this case we define two kinds of optimized squeezing spectra. One is obtained by minimizing the autocorrelation function in equation (43), with
, only over the phases of the local oscillators
; the other is obtained when the minimization also runs over the scaling parameters,
. In both cases they can be expressed in terms of the squeezing spectra resulting from the protocol described in section 4.3 as

Thus, according to equation (26), in the Gaussian case,
measures the entanglement between the modes whose operators are
and
.
5. Application to ponderomotive squeezing in a two-sided cavity
Here we study ponderomotive squeezing [43–46] and the conditions under which the spectral components of the field emitted by an optomechanical system are squeezed and entangled. Moreover we determine the squeezing spectra, and we identify the detectable spectral modes that exhibit maximum entanglement.
Ponderomotive squeezing refers to the squeezing of the output light resulting from the non-linear radiation-pressure interaction with a mechanical resonator inside an optical cavity. The response of a high-Q mechanical resonator to a resonance mode of a high-finesse optical cavity can be described as that of a Kerr medium, which imparts an intensity-dependent phase shift to the light. As a result the field fluctuations can be reduced, and correspondingly, squeezed light is produced [43, 44]. In detail, we investigate a Fabry–Perot cavity with a membrane in the middle [70]. A single optical mode is relevant in the system dynamics. It loses photons at rates
from the mirrors j = 1, 2 and is driven by a laser at a frequency detuned by δ from the relevant cavity resonance. Only one mechanical mode of the membrane at frequency
interacts significantly with the cavity field with a linearized coupling strength g. The decay rate of the membrane is γ, and the number of thermal mechanical excitations nT. The corresponding linearized optomechanical dynamics are Gaussian [47, 48] and are efficiently analyzed in terms of the standard input–output theory [69]. Here we describe the results for the field emitted through the two cavity mirrors at the steady state of the system dynamics in the regime of optomechanical stability, referring the reader appendix
The photons lost through the two cavity mirrors are described by the output field operators aout1,
, aout2, and
. The corresponding power spectrum matrix, defined in equation (9), can be evaluated for the vector of operators
, and the result is given by

where
is a diagonal matrix whose diagonal elements are
,
is a matrix whose only non zero elements are
,

and the matrix
is given in terms of the parameters

(with α complex even function of ω, and
real and positive) as

This matrix contains all the information about the spectral properties of the output fields and can be used to construct the correlation matrix for two spectral modes as in equation (15). In the following we will use this matrix and the results of sections 3 and 4 to study the corresponding entanglement properties.
5.1. Homodyne and heterodyne spectra and entangled components of the emitted field
In section 4 we described three different strategies for the experimental investigation of the spectral properties of stationary continuous fields, which are based on homodyne and heterodyne techinques. They probe different pairs of spectral modes given, respectively, by equations (30), (37), and (40). When applied to the investigation of the optomechanical system, these techniques allow the detection of the corresponding spectral components of the two output fields
, as depicted in figure 4. In particular, using these techniques it is possible to study composite quadratures of these pairs of modes and their squeezing and entanglement properties. We have identified two different kinds of optimized squeezing spectra, corresponding to different experimental approaches for the measurement and the minimization of the homodyne photocurrent fluctuations. Specifically, to probe symmetric superpositions of quadratures of the two modes it is sufficient to apply standard homodyne techniques; thus minimization is achieved by tuning the relative phase of the two quadratures, which is controlled experimentally by the phase of the local oscillator. We indicate this phase-optimized spectrum with the symbol
, where the label
is used to distinguish the three detection strategies (see figure 4). At the same time, non-symmetric superpositions, with different weights of the two quadratures, can be probed by combining different filtered photocurrents detected with appropriately selected phases of both the filter and the local oscillator. The globally optimized squeezing spectrum
is then obtained, minimizing the corresponding fluctuations over the phases of both the local oscillator and the filter.
Figure 4. Spectral components at the output of an optomechanical system that are probed with three different detection strategies and that are entangled, and squeezed, as a result of the optomechanical interaction.
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Standard image High-resolution imageIn all cases the squeezing spectra
and
are equal to equation (22) and (23), evaluated in each case for the specific parameters
and m, which correspond to the detected spectral modes. Specifically,
and
are obtained by the single-mode homodyne detection of a single field (either one of the two output fields), as discussed in section 4.1, and if applied to the output from the first mirror, then
and
. The second strategy is based on the two-mode homodyne detection of the two output fields (see section 4.2), and the corresponding spectra,
and
, are evaluated for
and
, where the operators
have the same form of equation (37), but in this case, they are constructed as the superpositions of the two filtered output fields
. Finally,
and
correspond to the two-mode heterodyne detection of the two output fields as discussed in section 4.4. If it is applied to the spectral component at frequency ω of the first output and at
of the second then
and
are evaluated for
and
. We note that these last two spectra can also be retrieved by combining various homodyne photocurrents as discussed in section 4.3.
The power spectrum matrix in equation (45) can be used to find

where

In the case of strategy
, the parameters
and
, in the expression for
, determine the specific detected composite modes, which are defined as in equation (37). We observe that when

then
; hence we can conclude that
evaluated for a two-sided configuration with decay rates
and
is equal to
when it is evaluated for a single-sided cavity with the decay rate equal to the sum of the decay rates
of the two-sided configuration. It indicates that the entanglement between
and
, in a single-sided cavity, is redistributed among the four spectral components
and
in the case of a two-sided cavity. For this reason, the same amount of squeezing found in the case of a single-sided cavity, can be recovered when the information from the two decay channels of a two-sided cavity are properly combined. In particular
is maximum for the parameters of equation (50) and consequently the corresponding modes are the collective modes that are maximally squeezed (and entangled).
We also note that according to equation (24) we find that, in all cases, the pairs of spectral components are entangled (and squeezed), although possibly with different degrees of entanglement (and squeezing), when

Moreover we note that the logarithmic negativity between the pair of spectral components detected with each strategy is obtained by applying the definition in equation (25) to the parameter

which is equal to the minimum symplectic eigenvalue of the corresponding partially transposed covariance matrix.
In figure 5 we compare the results for the spectra evaluated for realistic parameters and corresponding to the three detection strategies, and hence to different pairs of spectral components. Each plot in figure 5 is evaluated for different values of the relative decay rate
of the two mirrors, whereas the total decay rate
and all the other parameters are kept fixed. In plot (a) we study a single-sided cavity with
. In plot (b) the mirrors are lossy and non-symmetric, and finally in (c) the two mirrors are symmetric:
. When
, in plot (a), the curves for
,
,
, and
correspond to the situation in which the detector on the second mirror detects only vacuum fluctuations. It is therefore clear that the curves for
and
, which measure the correlations between the single spectral component
of the field lost from the first mirror and the single spectral component
of the field lost from the second show no squeezing. On the other hand, maximum two-mode squeezing and entanglement are observed for the single-mode homodyne spectra corresponding to the curves
and
, which measure the correlations between
and
. The curves
,
, that measure the correlations between the composite modes in equation (37), are at an intermediate value as a result of the vacuum fluctuations of the modes
, which reduces the visibility of the two-mode squeezing between
and
.
Figure 5. Squeezing spectrum
and symplectic eigenvalue
, obtained for the values of the decay rates of the cavity mirrors
and (a)
, (b)
, (c)
. In the insets the regions close to the upper mechanical resonance (
) are magnified. The other parameters are
,
,
, nT = 13091 (temperature = 100 mK and
MHz), and in the case of
and
, the spectral mode operators
are defined by the values
and
.
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Standard image High-resolution imagePlot (c) corresponds to a symmetric two-sided cavity with
. In this case the maximum squeezing and entanglement are obtained for the curves
and
, indicating that in this configuration the maximally entangled spectral components correspond to the composite modes in equation (37). In particular
and
are equal to the curves for
and
in the single-sided cavity reported in plot (a). In the two cases, the correlations of the cavity field built by the optomechanical dynamics are equal as a result of the equal total decay rate. The only difference is that, in one case all the photons are lost through a single mirror, whereas in the other they are split in the two decay channels and only their combined detection can reveal the corresponding total degree of squeezing and entanglement. Moreover in plot (c) we observe that
and
are equal to
and
. In this case, the two output fields are symmetric, hence the correlations between
and
are equal to those between
and
. Finally, plot (b) corresponds to an intermediate situation between the two described in (a) and (c), and it shows that the three detection strategies can display different degrees of squeezing. In general, the values of all the squeezing spectra can lie at any value between the extremes set by the corresponding curves in plot (a) and (c), depending on the actual value of the ratio
.
We also emphasize that the values of
and
are reported, in the three plots, for the same values of the parameters
and
which define the specific superposition of spectral components that are being probed as defined in equation (37). However, for each value of
the values of
and
can be appropriately tuned to find the composite modes that are characterized by the same maximum amount of squeezing as in plot (c). This is shown for the parameters of plot (b) and at
in figure 6, where maximum squeezing and entanglement (recovering the maximum value found in figure 5(c)) is found when
. We further observe that, in figure 5, the results for
and
are very close to
and
respectively. They are substantially different only close to the mechanical resonances (
), where, although the two spectral modes are entangled (
), this feature is not reflected in the corresponding squeezing spectrum
, which is significantly larger and very close to 1. This happens when the two corresponding spectral modes are significantly asymmetric so that
. This situation is realized very close to the condition
and for a bandwidth on the order of the mechanical dissipation rate γ, which, in a typical optomechanical system, can be very small, as shown in the insets of figure 5. On the other hand, the discrepancy between
and
can be considerably larger, covering, for example, the full spectrum in plots (a) and (b). This is because in this case the difference between the corresponding
and
is proportional to the difference between
and
, which is relatively large in plots (a) and (b). In plot (c), on the other hand, the two mirrors are symmetric and likewise
and
are very close, reproducing the results for
and
.
Figure 6. Squeezing spectrum
and symplectic eigenvalue
, as a function of the ratio
, when
,
,
,
,
,
, nT = 13091 (temperature = 100 mK and
MHz).
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Standard image High-resolution image6. Conclusions
In conclusion, we have presented a comprehensive analysis of the entanglement properties of stationary squeezed fields at the output of a quantum optical system. By revisiting a number of already known concepts and condensing them into a unified description, we have derived novel results that directly link the spectral properties of squeezed light fields, in the stationary continuous-wave regime, to the entanglement theory of continuous-variable systems. Specifically we have employed long-time filtered modes to systematically study the spectral properties of squeezed fields. Likewise we have derived general squeezing and entanglement criteria that are valid for stationary fields, and most important, we have established the equivalence between two-mode squeezing variance and logarithmic negativity for stationary Gaussian fields. In experiments, the squeezing properties of the field can be investigated with homodyne or heterodyne techniques. In particular the long time integration of the homodyne or heterodyne signal provides information about specific spectral components of the field and of the corresponding squeezing. We have analyzed the discrete bosonic operators describing such spectral modes and have studied the corresponding entanglement properties, thereby demonstrating that the measurable squeezing spectrum resulting from the spectral homodyne or heterodyne analysis of a field is indeed a direct measurement of the corresponding logarithmic negativity.
When applied to an optomechanical system comprising a two-sided Fabry–Perot cavity with a membrane in the middle, these findings help in identifying the specific spectral components of the output fields that are maximally entangled, showing, in particular, that maximum squeezing and entanglement are found between specific modes constituted by the superposition of carefully selected spectral components of the two outputs.
In general, a continuous-wave squeezed field combines, in a single spatial mode, a large number of spectral entangled sideband modes. It is, therefore, logical to ask whether and how one could exploit such a rich entanglement structure for real quantum-enhanced applications. Such a question has been addressed, for example, in [37–40], where it is discussed how to spatially separate the spectral sidebands of a continuous squeezed field to create N spatially independent entangled pairs and hence to prepare N quantum communication channels whose actual number is limited only by the spectral resolution of the experimental apparatus and by the bandwidth of the squeezed signal. In a similar perspective, it is intriguing to ask whether such a large number of entangled pairs could be exploited as a resource for frequency-encoded multimode entangled networks in the stationary continuous-wave regime, as an alternative to that achieved with pulsed frequency combs [18].
We finally remark that although here we have focused on spectral components, the approach based on the filtered modes that we have described in section 2.1 is sufficiently general to be applicable to a wider area of experimental situations in which finite-time filtered modes are relevant [61, 71–74].
Acknowledgments
This work has been supported by the European Commission (ITN–Marie Curie project cQOM and FET–Open Project iQUOEMS) and by MIUR (PRIN 2011).
Appendix A.: Squeezing and entanglement of discrete modes
Here we discuss some useful results regarding the squeezing and entanglement of discrete Gaussian modes [2, 75, 76]. Squeezing refers to the occurrence of reduced fluctuations of a quadrature of a field below the value of the fluctuations of a coherent state. Particularly interesting is two-mode squeezing, which refers to the squeezing of a combined quadrature of two modes, whereas the two separated modes are not squeezed. Two-mode squeezing is, in fact, a signature of entanglement between the two modes.
Let us now consider two discrete modes with annihilation operators, b1 and b2, for which
. Here and in the following, for simplicity, we assume that the average value of the fields is zero
, and only the fluctuations characterize the state of the two modes. A quadrature
is squeezed when the following relation is fulfilled:
. Two-mode squeezing is likewise found when the variance of a composite quadrature
is smaller than 1, i.e.,
. We note that this relation can be satisfied only if
. In general, two-mode squeezing variances of this form can be used to construct entanglement criteria. In particular, it was established [29], given a quadrature of the form

where
are real and positive. A sufficient condition for entanglement can be defined in terms of the quantity

Specifically, when
, for some values of
and
, the two modes are entangled. In the case of Gaussian fields this criterion also becomes a necessary condition for entanglement (for appropriate values of
) [2].
In the analysis of the entanglement properties of Gaussian systems, for which all the information is contained in the first and second moments of the field operators, it is useful to introduce the following matrix notation. We consider the column vector of operators
and the corresponding correlation matrix, which is given by

whose elements are
. The corresponding covariance matrix, C, namely the symmetric matrix of correlations of the quadrature
and
, can be used to compute entanglement measures, such as the logarithmic negativity. It is given by
, where we have introduced the matrix

The logarithmic negativity for Gaussian states is then computed as
, where ν is the smallest symplectic eigenvalue of the covariance matrix of the partially transposed state that can be expressed as
, where Π is a diagonal matrix whose diagonal elements are
[62]. In particular, this relation implies that the state is entangled when
.
A generic covariance matrix can always be transformed, using only local symplectic transformation, into the standard form [29]

where a, b, c and c' are reals. In this case the corresponding matrix of correlations for the field operators reads

where

The symplectic eigenvalue ν in the definition of the logarithmic negativity can be expressed in terms of the elements of these matrices as

Likewise, these matrices can be used to determine an explicit expression for ES

that is minimized for

and the corresponding minimum is

We note that if
(i.e.,
), then
is equal to equation (A.8), that is,

This result is important because it directly joins an entanglement measure, namely the logarithmic negativity, to the field observables, namely the variances of the field quadratures. As we have seen, this is true only for the specific class of states for which
that correspond to the condition
with
(or equivalently
). A related result was previously discussed in [77], where the symplectic eigenvalue was shown to be equal to the EPR correlations in the case of symmetric states, for which a = b.
As discussed in the main text, the condition
is relevant to the study of entanglement between the spectral components of stationary continuous fields. The general corresponding correlation matrix takes the form of equation (16), for which the correlations of the form
are zero. We note that in this case equation (A.6) is equal to twice equation (22) when
and
, where
is the phase of the complex parameter m, which is introduced in equation (16). The minimization of equation (22) is therefore similar to equations (A.7) and (A.8) (see equation (23)). The corresponding covariance matrix is given by

We note that this matrix and the matrix in equation (16) are not, in general, in the standard form described by equations (A.3) and (A.4). They can be cast in standard form by means, for example, of the single-mode rotation that performs the transformation
. Thus the resulting matrices are equal to equations (A.3) and (A.4), with
and
. Therefore the corresponding minimum symplectic eigenvalue of the partially transposed covariance matrix has the form of equation (A.5) with
and
, and it is explicitly given by equations (23) and (26).
Appendix B.: The power spectrum of the stationary homodyne/heterodyne photocurrent
In homodyne and heterodyne detection techniques [5, 41, 64–67] the signal field is mixed on a 50:50 beam splitter with a strong monochromatic field at the frequency
, the local oscillator. When the frequency of the local oscillator is equal to the carrier frequency,
, then one has homodyne detection. Heterodyne detection corresponds, instead, to finite detuning
. The fields at the two output ports of the beam splitter are detected and the corresponding photo-currents are subtracted to end up with a classical electronic signal (which contains informations about a particular quadrature of the signal field):

where
is a classical random variable and θ is the phase of the local oscillator, with
corresponding to homodyne detection. Information about the spectral components of a detected stationary signal are provided by the power spectrum that quantifies the strength of the fluctuations at specific frequencies. We will refer to it as the homodyne or heterodyne spectrum. It is given by

where here the angular brackets need to be intended as ensemble averages over many experimental runs and where we use the fact that the photocurrent is a real stationary random process, for which the two-times correlation function depends only on the time difference and is symmetric
. In particular this implies that

The power spectrum can be equivalently expressed trough the relation

where
. In practice the homodyne/heterodyne spectrum is evaluated in an approximate way by filtering the photocurrent with a filter function of length τ:

and then calculating the corresponding autocorrelation function,

When τ is sufficiently large, the spectral properties of the stationary signal can be resolved and the power spectrum is well approximated

This relation can be demonstrated as follows. The filtered photocurrent is equivalently given by

where the filter function
is defined in equation (7). Thus we find

where we have used equation (B.4). In the large τ limit the modulus square of the filter function is equal to a delta function, yielding therefore equation (B.7).
We remark that the filtered photocurrent in equation (B.5) is complex and therefore is not directly related to a measurable (real) quantity. However, we note that the same result presented in equation (B.7) is obtained if, instead, we use the real photocurrent

In particular the corresponding power spectrum is independent of the phase φ. To demonstrate this statement we rewrite equation (B.10) as

Hence the corresponding autocorrelation function is given by

where we have used the relation
and equation (B.4). Finally, using equations (12) and (B.3) we find that, in the limit of large τ, this equation reduces to equation (B.7).
The photocurrent is directly related to the properties of the detected field. In fact, the ensemble average in equation (B.2) can be equivalently interpreted as a quantum average over an operator of the form

where now a(t) and
are quantum operators for the detected field and the results discussed earlier, in terms of classical photocurrents, can be straightforwardly rephrased in terms of this quantum operator.
Furthermore, although the results for the homodyne and heterodyne spectra are independent of the form of the filtered photocurrent, whether equation (B.5) or (B.10), the choice of equation (B.10) is physically motivated by the fact that it results in a real filtered photocurrent that corresponds to a Hermitian quantum operator, and hence it makes transparent the relation between the spectral properties of the detected photocurrent and the corresponding quantum observables of the stationary field. In particular the filtered photocurrent can be described by the Hermitian operator

where the normalization factor
is appropriately chosen to satisfy the commutation relation for quadrature operators
, namely
. Thus, the filtered photocurrent can be expressed as the sum of two filtered quadrature operators for the two frequency bands of width
each, centered at the frequencies
,

where

with the annihilation operator, of a single-band filtered mode, defined as in equation (4). In the limit of large τ, equation (B.14) reduces to equations (29) and (41), when, respectively,
and
.
Appendix C.: A single-mode cavity with a membrane in the middle: Input–output theory
We consider a single-mode Fabry–Perot cavity with a membrane in the middle as discussed in the main text. The quantum Langevin equations [78] for the creation and annihilation operators of a cavity photon
and of a membrane phonon
, in the linearized regime [47] can be expressed in matrix form as

where
is the column vector of system operators
, the matrix of coefficients
is given by

with the parameters defined in the main text, and
is the vector of input noise operators
, which includes the two inputs of the cavity corresponding to the two mirrors. Finally
, is the 4 × 6 matrix

In general the system dynamics can be divided into two main parameter regimes [47]. When the real part of all the eigenvalues of the matrix
is negative, the system is stable and approaches a steady state at long times. If, on the other hand, some eigenvalues have a positive real part, the system is not stable, the populations of the modes explode, and no steady state is reached. In this second case the linearized model in equation (C.1) is not a valid description of the optomechanical dynamics. All the results presented in the main text correspond to the regime of optomechanical stability.
The steady state corresponding to equation (C.1) can be easily obtained in Fourier space. We introduce the Fourier-transformed operators
, hence

We are interested in the field leaking out by the two cavity mirrors. According to the input–output theory [78], the operators for the output fields can be expressed in terms of the system and of the input noise operators as
, where j = 1, 2 distinguish the two output channels corresponding to the two cavity mirrors. To express these relations in matrix form we introduce the 4 × 6 matrix

that when applied to the vector of input operators gives
and selects only the noise operators corresponding to the two output channels. Thus, the vector of output operators
can be written as

Using equation (C.4) we find

and the corresponding power spectrum matrix is

where
is the correlation matrix of the input noise operators defined as
, and it is given by

where nT is the number of thermal excitations of the mechanical oscillator. The explicit result for
is given in equation (45).





