The broadband Raman conversion of femtosecond-light pulses to the anti-Stokes side is demonstrated. A 130 fs light pulse from a Ti:sapphire-based regenerative amplifier system is divided into two light pulses. They are focused on a SrTiO3 crystal with a finite cross angle. Over 24 higher-order coherent anti-Stokes Raman scattering signals are observed, which cover from near infrared to green. These higher-order coherent anti-Stokes Raman scattering (CARS) signals come from the resonant excitation of two-phonon waves. The results offer a possibility of an all solid-state anti-Stokes Raman shifter covering an extremely broadband tunable range.