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The statistics of collapsing square lattice trails with a fixed number of vertices of degree 4

E W James1 and C E Soteros2

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A trail on the square lattice with a fixed number, k, of vertices of degree 4 is called a k-trail. We model polymer collapse using k-trails by incorporating an interaction energy which is proportional to the number of nearest-neighbour contact edges of the trail. It is known that the number of square lattice n-edge closed (open) k-trails can be bounded above and below (to O(nk)) by the number of n-step self-avoiding circuits (walks). This along with pattern theorems for self-interacting self-avoiding circuits and walks are used herein to establish upper and lower bounds (to O(nk)) for the collapsing free energy of k-trails in terms of self-avoiding circuits or walks, as appropriate. We also use pattern theorems to obtain bounds on the limiting nearest-neighbour contact density for collapsing k-trails. Finally, we investigate k-trails with a fixed density of nearest-neighbour contacts and show that their limiting entropy per monomer is independent of k.


PACS

05.50.+q Lattice theory and statistics (Ising, Potts, etc.)

05.40.Fb Random walks and Levy flights

61.25.H- Macromolecular and polymers solutions; polymer melts

MSC

82B41 Random walks, random surfaces, lattice animals, etc. (See also 60G50, 82C41)

82D60 Polymers

Subjects

Soft matter, liquids and polymers

Statistical physics and nonlinear systems

Dates

Issue 50 (14 December 2007)

Received 1 September 2007, in final form 24 October 2007

Published 28 November 2007



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