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Research in aerosol properties and cloud characteristics have
historically been considered two separate disciplines within the
field of atmospheric science. As such, it has been uncommon for a
single researcher, or even research group, to have considerable
expertise in both subject areas. The recent attention paid to
global climate change has shown that clouds can have a considerable
effect on the Earth's climate and that one of the most uncertain
aspects in their formation, persistence, and ultimate dissipation
is the role played by aerosols. This highlights the need for
researchers in both disciplines to interact more closely than they
have in the past. This is the vision behind this focus issue of
Environmental Research Letters.
Certain interactions between aerosols and clouds are relatively
well studied and understood. For example, it is known that an
increase in the aerosol concentration will increase the number of
droplets in warm clouds, decrease their average size, reduce the
rate of precipitation, and extend the lifetime. Other effects are
not as well known. For example, persistent ice super-saturated
conditions are observed in the upper troposphere that appear to
exceed our understanding of the conditions required for cirrus
cloud formation. Further, the interplay of dynamics versus effects
purely attributed to aerosols remains highly uncertain. The purpose
of this focus issue is to consider the current state of knowledge
of aerosol/cloud interactions, to define the contemporary
uncertainties, and to outline research foci as we strive to better
understand the Earth's climate system.
This focus issue brings together laboratory experiments, field
data, and model studies. The authors address issues associated with
warm liquid water, cold ice, and intermediate temperature
mixed-phase clouds. The topics include the uncertainty associated
with the effect of black carbon and organics, aerosol types of
anthropogenic interest, on droplet and ice formation. Phases of
water which have not yet been fully defined, for example cubic ice,
are considered. The impact of natural aerosols on clouds, for
example mineral dust, is also discussed, as well as other natural
but highly sensitive effects such as the
Wegener–Bergeron–Findeisen process.
It is our belief that this focus issue represents a leap forward
not only in reducing the uncertainty associated with the
interaction of aerosols and clouds but also a new link between
groups that must work together to continue progress in this
important area of climate science.
Focus on Aerosol–Cloud Interactions Contents
The global influence of dust
mineralogical composition on heterogeneous ice nucleation in
mixed-phase clouds
C Hoose, U Lohmann, R Erdin and I Tegen
Ice formation via deposition
nucleation on mineral dust and organics: dependence of onset
relative humidity on total particulate surface area
Zamin A Kanji, Octavian Florea and Jonathan P D Abbatt
The Explicit-Cloud
Parameterized-Pollutant hybrid approach for aerosol–cloud
interactions in multiscale modeling framework models: tracer
transport results
William I Gustafson Jr, Larry K Berg, Richard C Easter and
Steven J Ghan
Cloud effects from boreal forest
fire smoke: evidence for ice nucleation from polarization lidar
data and cloud model simulations
Kenneth Sassen and Vitaly I Khvorostyanov
The effect of organic coating on
the heterogeneous ice nucleation efficiency of mineral dust
aerosols
O Möhler, S Benz, H Saathoff, M Schnaiter, R Wagner, J
Schneider, S Walter, V Ebert and S Wagner
Enhanced formation of cubic ice in
aqueous organic acid droplets
Benjamin J Murray
Quantification of water uptake by
soot particles
O B Popovicheva, N M Persiantseva, V Tishkova, N K Shonija and N
A Zubareva
Meridional gradients of light
absorbing carbon over northern Europe
D Baumgardner, G Kok, M Krämer and F Weidle
MAID: a model to simulate UT/LS
aerosols and ice clouds
H Bunz, S Benz, I Gensch and M Krämer
Single-parameter estimates of
aerosol water content
S M Kreidenweis, M D Petters and P J DeMott
Supersaturations, microphysics and
nitric acid partitioning in a cold cirrus cloud observed during
CR-AVE 2006: an observation–modelling intercomparison
study
I V Gensch, H Bunz, D G Baumgardner, L E Christensen, D W Fahey,
R L Herman, P J Popp, J B Smith, R F Troy, C R Webster, E M
Weinstock, J C Wilson, T Peter and M Krämer
Connecting hygroscopic growth at
high humidities to cloud activation for different particle
types
H Wex, F Stratmann, T Hennig, S Hartmann, D Niedermeier, E
Nilsson, R Ocskay, D Rose, I Salma and M Ziese
Modeling of the
Wegener–Bergeron–Findeisen process—implications
for aerosol indirect effects
T Storelvmo, J E Kristjánsson, U Lohmann, T Iversen, A
Kirkevåg and Ø Seland
Droplet nuclei in non-precipitating
clouds: composition and size matter
Cynthia H Twohy and James R Anderson
A laboratory investigation of the
relative humidity dependence of light extinction by organic
compounds from lignin combustion
Melinda R Beaver, Rebecca M Garland, Christa A Hasenkopf,
Tahllee Baynard, A R Ravishankara and Margaret A Tolbert
Cirrus cloud formation and ice
supersaturated regions in a global climate model
Ulrike Lohmann, Peter Spichtinger, Stephanie Jess, Thomas Peter
and Herman Smit
Notes on state-of-the-art
investigations of aerosol effects on precipitation: a critical
review
A P Khain