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Structure of spinel at high temperature using in-situ XANES study at the Al and Mg K-edge

D de Ligny1, D R Neuville2, A-M Flank3 and P Lagarde3

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We present structural information obtained on spinel at high temperature (298–2400 K) using in situ XANES at the Mg and Al K-edge. Spinel, [4](Alx,Mg1-x)[6](Al2-x,Mgx)O4, with increasing temperature, show a substitution of Mg by Al and Al by Mg in their respective sites. This substitution corresponds to an inversion of the Mg and Al sites. Furthermore, both experiments at the Al and Mg K-edges are in good agreement with XANES calculation made using FDMNES code.


PACS

78.70.Dm X-ray absorption spectra

61.66.Fn Inorganic compounds

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 1 (2009)



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