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In-situ investigation of Bi thin film condensation by surface sensitive X-ray absorption spectroscopy at cryogenic temperatures

D Lützenkirchen-Hecht, C Markert, R Wagner and R Frahm

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Reflection mode grazing incidence X-ray absorption spectroscopy at the Bi L3-edge and simultaneous electrical resistivity measurements were used to investigate the microstructure of quench condensed thin Bi metal films on float-glass substrates at temperatures from 20 K to 300 K. While thin films of ≈ 6 nm thickness appear to be amorphous after deposition at 20 K, thicker films of about 18 nm show the well-known rhombohedral structure of bulk Bi. During a subsequent heat treatment, the amorphous structure of the thin films transforms irreversibly into the crystalline form for temperatures at (42 ± 2) K. This crystallisation is accompanied by an irreversible increase of the film resistivity by a factor of more than 2.7. The film density and roughness do not change within detection limits during the heat treatment.


PACS

78.70.Dm X-ray absorption spectra

61.43.Dq Amorphous semiconductors, metals, and alloys

81.40.Gh Other heat and thermomechanical treatments

68.55.-a Thin film structure and morphology

73.61.At Metal and metallic alloys

Subjects

Condensed matter: electrical, magnetic and optical

Semiconductors

Surfaces, interfaces and thin films

Condensed matter: structural, mechanical & thermal

Dates

Issue 1 (2009)



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