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Iodine K-edge EXAFS analysis of iodide ion-cyclodextrin inclusion complexes in aqueous solution

T Kaneko1, M Ueda2, S Nagamatsu2, T Konishi2, T Fujikawa2 and M Mizumaki3

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We study the structure of inclusion complexes of α-, β-, γ-cyclodextrin with mono-iodide ion in aqueous solution by means of iodine K-edge EXAFS spectroscopy. The analysis is based on the assumption that two kinds of iodide ions exist in KI-cyclodextrin aqueous solution i.e. hydrated mono-iodide ions and one-one mono-iodide-cyclodextrin inclusion complexes. In KI-α-cyclodextrin system, iodine K-edge EXAFS analyse show that the average coordination number of the oxygen atoms in water molecules in the first hydration shell decreases as the fraction of included ions increases. This result suggests that dehydration process accompanies the formation of the inclusion complex. This is not found in the case of β-cyclodextrin, indicating that in this case the iodide ions are included together with the whole first hydration shell.


PACS

78.70.Dm X-ray absorption spectra

61.25.Em Molecular liquids

82.30.-b Specific chemical reactions; reaction mechanisms

Subjects

Soft matter, liquids and polymers

Condensed matter: electrical, magnetic and optical

Chemical physics and physical chemistry

Dates

Issue 1 (2009)



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