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1H-NMR study of the idle-spin magnet Cu3(OH)4SO4

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, , Citation Y Fujii et al 2009 J. Phys.: Conf. Ser. 145 012061 DOI 10.1088/1742-6596/145/1/012061

1742-6596/145/1/012061

Abstract

1H-NMR study of a spin-1/2 triple-chain system Cu3(OH)4SO4, in which the realization of an `idle-spin' state has been suggested recently from neutron experiments, were carried out in the temperature range down to 1.4 K. In the experiments under about 1 T, we found a clear anomaly of the nuclear magnetic relaxation rate and drastic change of the spectrum at around TN = 5.4 K. NMR spectrum below TN has a characteristic shape of an antiferromagnetic ordered state. This low-temperature spectrum is consistently reproduced by the calculation of local fields at proton sites on the basis of the idel-spin state. Further, TN decreased as the applied field is increased up to 6.9 T.

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10.1088/1742-6596/145/1/012061