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Ab initio investigations of the charge transport properties of endohedral M@C20 (M = Na and K) metallofullerenes

An Yi-Peng (安义鹏)1, Yang Chuan-Lu (杨传路)1,2, Wang Mei-Shan (王美山)1, Ma Xiao-Guang (马晓光)1 and Wang De-Hua (王德华)1

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Using density functional theory and quantum transport calculations based on nonequilibum Green's function formalism, we investigate the charge transport properties of endohedral M@C20(M = Na and K) metallofullerenes. Our results show that the conductance of C20 fullerene can be obviously improved by insertion of alkali atom at its centre. Both linear and nonlinear sections are found on the I—V curves of the Au-M@C20-Au two-probe systems. The novel negative differential resistance behaviour is also observed in Na@C20 molecule but not in K@C20.


PACS

71.20.Tx Fullerenes and related materials; intercalation compounds

72.80.Rj Fullerenes and related materials

71.15.Mb Density functional theory, local density approximation, gradient and other corrections

Subjects

Condensed matter: electrical, magnetic and optical

Dates

Issue 11 (November 2010)

Received 1 March 2010, in final form 6 March 2010



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