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Enhanced atomic Kerr nonlinearity in bright coherent states

A M Akulshin, A I Sidorov, R J McLean and P Hannaford

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We show that long-lived bright Zeeman coherence that is responsible for absorption enhancement and steep anomalous dispersion in an atomic medium gives rise to a giant nonlinearity of the atomic susceptibility, in a similar manner to the dark coherence responsible for the well-known electromagnetically induced transparency. The intensity dependent refractive index of Cs vapour with a ground state Zeeman coherence in the vicinity of the D2 resonance line has been measured at low light intensity. The Kerr nonlinearity in the bright coherent state (n2 ≈ 1.0 × 10-6 cm2 mW-1) is higher than that in a dark state under the same experimental conditions. Higher order nonlinear components of the refractive index have also been estimated for both coherent states.


PACS

42.65.Hw Phase conjugation; photorefractive and Kerr effects

32.60.+i Zeeman and Stark effects

42.50.Gy Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption

42.50.Md Optical transient phenomena: quantum beats, photon echo, free-induction decay, dephasings and revivals, optical nutation, and self-induced transparency

42.65.An Optical susceptibility, hyperpolarizability

Subjects

Atomic and molecular physics

Optics, quantum optics and lasers

Dates

Issue 12 (December 2004)

Received 18 August 2004, accepted for publication 8 October 2004

Published 15 October 2004



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