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Third-harmonic generation and laser-induced continuum structure in sodium

K G H Baldwin1,4, M D Bott2, H-A Bachor2 and P B Chapple3

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Observation of laser-induced continuum structure (LICS) in sodium due to the coupling of a bound state to the continuum by a strong laser field has been reported elsewhere. Such experiments have mostly employed a single laser photon to probe the structured continuum from the ground state. Other experiments have used multiphoton (third harmonic) probe schemes, but only one of these has successfully observed LICS, in agreement with theoretical predictions. We report here a very similar experiment generating third-harmonic radiation in sodium to probe the anticipated LICS produced by coupling the 5s state to the p continuum. However, under no conditions was any continuum structure observed, in agreement with in a number of other experiments, but at variance with theoretical predictions.


PACS

42.65.Ky Frequency conversion; harmonic generation, including higher-order harmonic generation

42.50.Hz Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift

42.60.Fc Modulation, tuning, and mode locking

42.60.Jf Beam characteristics: profile, intensity, and power; spatial pattern formation

42.60.Lh Efficiency, stability, gain, and other operational parameters

Subjects

Optics, quantum optics and lasers

Dates

Issue 4 (August 2000)

Received 21 March 2000



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