Frontiers of muon spectroscopy—25 years of muon science at ISIS

The ISIS muon source developed with support from the European Community (EC) and groups at Grenoble, Parma, Uppsala and Munich in the late 1980s, with a single instrument providing many scientists with their first opportunity to explore the unique capabilities of muon spectroscopy. The timing was opportune, as the muon technique was making an important contribution to the study of the then recently discovered cuprate high T_c superconductors. The ISIS user community developed rapidly over subsequent years, with the technique finding a broad range of applications in condensed matter physics, materials science and chemistry. The single instrument was hugely oversubscribed, and the importance of the technique was recognized in 1993 with a further grant from the EC to develop the triple beamline facility that is currently available at ISIS. During 2009 the suite of spectrometers available at the facility received a major upgrade, with the Science and Technology Facilities Council funding the development of a 5 T high field instrument that has enabled entirely new applications of muon spectroscopy to be explored. The facility continues to flourish, with a strong user community exploiting the technique to support research across an increasingly broad range of subject areas. Condensed matter science continues to be a major area of interest, with applications including semiconductors and dielectrics, superconductors, magnetism, interstitial diffusion and charge transport. Recently, however, molecular science and radical chemistry have become prominent in the ISIS programme, applications where the availability of high magnetic fields is frequently vital to the success of the experiments.

For ISIS, 23 March 2012 marked a significant milestone, it being 25 years since muons were first produced at the facility for research in condensed matter and molecular science. To celebrate, the ISIS muon group organized a science symposium with the theme 'Frontiers of Muon Spectroscopy' at St Hugh's College, Oxford, UK during the autumn of 2012. While in part a retrospective, the focus of the meeting was on the state of the art, considering how muon techniques continue to contribute across many topical areas of research, with a forward look at new applications of the method. I should take this opportunity to thank the ISIS user community for their support for this meeting, and contributing to the diverse and interesting programme that was enjoyed by those attending. While a short account of the meeting and many of the presentations can be found on the group website at www.isis.stfc.ac.uk/groups/muons/meetings/, I am particularly grateful to Physica Scripta for giving the community the opportunity to publish a series of extended papers developing topics discussed during the meeting. Although many appear within this issue, the Swedish contribution will be published later, in 2014, as part of a series commemorating Swedish neutron and muon research at ISIS. I commend these papers to you; together they provide an excellent account of the technique and its unique role in many topical areas of research.

The symposium also marked the recent retirement of Professor Steve Cox. Steve has been involved with the muon technique for over 30 years, contributing to the development of muon science at ISIS throughout the life of the facility. During this time his research interests have embraced most areas of muon spectroscopy with a particular focus on applications in chemical physics, aspects of semiconductor science and muonium chemistry. He developed a keen interest in using muons to investigate elemental materials, publishing a major report looking at muonium as a model for interstitial hydrogen in the semiconducting and semimetallic elements [1], with further work focused on establishing the nature of the elusive muonium centre in sulphur [2]. In parallel, Steve continued to lead work looking at hydrogen defect centres in narrow-gap oxide semiconductors as a model for understanding the role of hydrogen in these materials, work that led to two major publications [3, 4].

References

[1] Cox S F J 2009 Rep. Prog. Phys. 72 116501

[2] Cox S F J et al 2011 J. Phys.: Condens. Matter 23 315801

[3] Cox S F J et al 2006 J. Phys.: Condens. Matter 18 1061

[4] Cox S F J et al 2006 J. Phys.: Condens. Matter 18 1079