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Deutsche Physikalische Gessellschaft IOP Institute of Physics

Ultrafast optical excitations of metallic nanostructures: from light confinement to a novel electron source

Focus on Advances in Surface and Interface Science

Claus Ropers1, Thomas Elsaesser1, Giulio Cerullo2, Margherita Zavelani-Rossi2 and Christoph Lienau3,4

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Part of Focus on Advances in Surface and Interface Science

Combining ultrafast coherent spectroscopy with nano-optical microscopy techniques offers a wealth of new possibilities for exploring the structure and function of nanostructures. In this paper, we describe newly developed nano-optical methods based on short-pulse laser sources with durations in the 10 fs regime. These techniques are used to unravel some of the intricate dynamics of elementary excitations in metallic nanostructures. Specifically, we explore light localization and storage in plasmonic crystals, demonstrate field enhancement and second harmonic generation from metallic nanotips and describe a novel nanometre-sized source of electron pulses. The rapid progress in this area offers exciting new prospects for probing and controlling electron dynamics in metallic nanostructures with femtosecond temporal and nanometre spatial resolution.


PACS

78.67.-n Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures

78.47.-p Spectroscopy of solid state dynamics

42.65.Ky Frequency conversion; harmonic generation, including higher-order harmonic generation

73.20.Mf Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Optics, quantum optics and lasers

Nanoscale science and low-D systems

Dates

Issue 10 (October 2007)

Received 4 June 2007

Published 31 October 2007



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