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Deutsche Physikalische Gessellschaft IOP Institute of Physics

Electron states and the spin density wave phase diagram in Cr(1 1 0) films

Focus on Photoemission and Electronic Structure

Eli Rotenberg1, B K Freelon1, H Koh1, A Bostwick1, K Rossnagel1, Andreas Schmid2 and S D Kevan3

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Part of Focus on Photoemission and Electronic Structure

Chromium films offer an excellent system to study the impact of dimensional confinement on physical properties associated with the spin-density-wave (SDW) ground state observed in bulk materials. These properties are also of some technological importance since chromium is a common component of thin film magnetic structures. We prepared chromium (1 1 0) films of high crystalline quality on a W(1 1 0) substrate with a wedge-shaped thickness profile so that the impact of confinement can be systematically studied. We have characterized these films using a combination of low-energy electron diffraction and microscopy as well as high-resolution angle-resolved photoemission spectroscopy. We have probed the Fermi surface and the nesting vectors therein that are relevant to the SDW ground state. We find these to predict accurately the observed bulk SDW periodicity. We have also characterized the SDW periodicity in the film directly by measuring the splitting between backfolded bands, and we find that this periodicity deviates markedly from the bulk periodicity for thinner films at higher temperatures. We have systematically mapped the SDW incommensurability and phase diagram as a function of both film thickness and temperature. We find commensurate and incommensurate phases that are separated by nearly continuous transitions. Our results suggest a simple model to explain the delicate interplay between commensurate and incommensurate phases that involves a balance between SDW stabilization energy and surface and interface energetics.


PACS

71.20.Be Transition metals and alloys

68.55.-a Thin film structure and morphology

64.70.Rh Commensurate-incommensurate transitions

75.30.Fv Spin-density waves

71.18.+y Fermi surface: calculations and measurements; effective mass, g factor

79.60.Dp Adsorbed layers and thin films

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Condensed matter: structural, mechanical & thermal

Dates

Issue 1 (April 2005)

Received 20 January 2005

Published 29 April 2005



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