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Deutsche Physikalische Gessellschaft IOP Institute of Physics

Attosecond pulse generation from aligned molecules—dynamics and propagation in H2+

Focus on Attosecond Physics

E Lorin1,3, S Chelkowski2 and A D Bandrauk1,2

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Part of Focus on Attosecond Physics

The dynamics and propagation effects in attosecond (asec) pulse generation from high-order harmonic generation (HHG) of aligned one-dimensional (1D) H2+ molecules are investigated from numerical solutions of fully coupled Maxwell and time-dependent Schrödinger equations (Maxwell-TDSEs), in the highly nonlinear nonperturbative regime of laser–molecule interaction. Density, laser-phase and propagation length effects are studied on the total electric field and nonlinear polarization from the Maxwell-TDSE for intense few cycle (800 nm) laser pulses interacting with a 1D H2+ gas. We show how single and double asec pulses can be generated and propagated as a function of the phase of individual harmonics created by ultrashort intense laser pulses in aligned H2+ molecules. We find furthermore extension of maximum HHG plateaux with increasing gas pressure.


PACS

33.80.-b Photon interactions with molecules

31.15.xv Molecular dynamics and other numerical methods

Subjects

Atomic and molecular physics

Computational physics

Dates

Issue 2 (February 2008)

Received 17 September 2007

Published 29 February 2008



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