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Deutsche Physikalische Gessellschaft IOP Institute of Physics

Broadband generation in a Raman crystal driven by a pair of time-delayed linearly chirped pulses

Focus on Attosecond Physics

Miaochan Zhi1 and Alexei V Sokolov

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Part of Focus on Attosecond Physics

A pair of time-delayed linearly chirped pulses with sub-picosecond duration is used to selectively excite Raman transitions in a lead tungstate crystal. Significant molecular coherence leads to generation of up to 40 anti-Stokes and 5 Stokes sidebands. High conversion efficiency (from the two pump beams to the sidebands) is measured. The broadband generation with chirped pulses whose duration is comparable to the Raman coherence lifetime is considerably more efficient, when compared to the case of excitation by two-color femtosecond pulses. In the future, mutual coherence among the generated sidebands may allow ultrashort pulse synthesis.


PACS

42.55.Rz Doped-insulator lasers and other solid state lasers

42.60.Fc Modulation, tuning, and mode locking

42.55.Ye Raman lasers

42.60.Jf Beam characteristics: profile, intensity, and power; spatial pattern formation

42.65.Re Ultrafast processes; optical pulse generation and pulse compression

42.70.Hj Laser materials

Subjects

Optics, quantum optics and lasers

Dates

Issue 2 (February 2008)

Received 19 October 2007

Published 29 February 2008



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