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Deutsche Physikalische Gessellschaft IOP Institute of Physics

Quantum-path control in high-order harmonic generation at high photon energies

Focus on Attosecond Physics

Xiaoshi Zhang1, Amy L Lytle, Oren Cohen, Margaret M Murnane and Henry C Kapteyn

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Part of Focus on Attosecond Physics

We show through experiment and calculations how all-optical quasi-phase-matching of high-order harmonic generation can be used to selectively enhance emission from distinct quantum trajectories at high photon energies. Electrons rescattered in a strong field can traverse short and long quantum trajectories that exhibit differing coherence lengths as a result of variations in intensity of the driving laser along the direction of propagation. By varying the separation of the pulses in a counterpropagating pulse train, we selectively enhance either the long or the short quantum trajectory, and observe distinct spectral signatures in each case. This demonstrates a new type of coupling between the coherence of high-order harmonic beams and the attosecond time-scale quantum dynamics inherent in the process.


PACS

42.65.Ky Frequency conversion; harmonic generation, including higher-order harmonic generation

Subjects

Optics, quantum optics and lasers

Dates

Issue 2 (February 2008)

Received 3 October 2007

Published 29 February 2008



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