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Kinetics of fission product gas release during grain growth

K Forsberg1 and A R Massih2,3,4

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A theoretical framework for the calculation of fission product gas release by diffusion, irradiation-induced re-solution, grain boundary saturation and grain growth in ceramic nuclear fuel (UO2) under time-varying loads is presented. The diffusion equation is subjected to boundary conditions, which account for the aforementioned effects. Analytical solutions to the equation are obtained. The theory is applied to calculate fission gas release and grain growth as functions of temperature and time. Correlation between grain growth and gas release is calculated and the results are discussed in the light of experimental data.


PACS

28.41.Bm Fuel elements, preparation, reloading, and reprocessing

66.30.-h Diffusion in solids

61.72.Mm Grain and twin boundaries

28.50.-k Fission reactor types

81.30.-t Phase diagrams and microstructures developed by solidification and solid–solid phase transformations

Subjects

Nuclear physics

Condensed matter: structural, mechanical & thermal

Dates

Issue 3 (April 2007)

Received 11 July 2006, in final form 31 January 2007

Published 26 March 2007



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