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Microwave-assisted synthesis of Sb2Se3 submicron rods, compared with those of Bi2Te3 and Sb2Te3

Bo Zhou1,2 and Jun-Jie Zhu2,3

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Orthorhombic Sb2Se3 submicron rods were prepared from antimony sodium tartrate and Se powder via a microwave-assisted chemical method. The products were characterized by x-ray powder diffraction (XRD), transmission electron microscope (TEM) and selected-area electron diffraction (SAED) techniques. The reaction mechanism and the morphology of the product were studied in detail in comparison with those in the syntheses of Bi2Te3 and Sb2Te3. The synthesis of Sb2Se3 was based on the polyol reducing process and microwaves played an important role. The morphologies of the compounds were mainly determined by their inherent anisotropic crystal structures. The optical properties of as-prepared Sb2Se3 were also characterized by UV–vis diffuse reflectance spectroscopy, and the bandgap (Eg) can be derived to be 1.16 eV, which is suitable for applications in photovoltaic conversion.


PACS

81.16.Be Chemical synthesis methods

81.07.-b Nanoscale materials and structures: fabrication and characterization

73.22.-f Electronic structure of nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals

61.46.-w Structure of nanoscale materials

78.40.Fy Semiconductors

78.67.-n Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures

Subjects

Condensed matter: electrical, magnetic and optical

Semiconductors

Nanoscale science and low-D systems

Dates

Issue 8 (25 February 2009)

Received 31 October 2008, in final form 12 December 2008

Published 2 February 2009



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