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Small-angle scattering investigations of Mg-borohydride infiltrated in activated carbon

Sabrina Sartori1,3, Kenneth D Knudsen1, Zhirong Zhao-Karger2, Eisa Gil Bardaij2, Maximilian Fichtner2 and Bjørn C Hauback1

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One of the main challenges for introduction of a hydrogen-based economy is storage of hydrogen. Hydrogen storage in solid materials is considered among the most attractive methods. During recent years much emphasis has been placed on the synthesis of nanosized metals and alloys. In the present study Mg(BH4)2 and Mg(11BD4)2 are infiltrated in pre-treated activated carbon and investigated with small-angle neutron scattering (SANS). The infiltration method is shown to be successful in modifying the size of the Mg-borohydride particles, as confirmed by scanning electron microscopy and x-ray diffraction data. The size of the particles for the infiltrated samples is estimated by SANS measurements to be mainly in the range <4 nm. The results suggest that the smallest pores of the scaffold are partially or fully filled and that this type of scaffold acts as an effective dispersing agent for Mg-borohydride.


PACS

84.60.-h Direct energy conversion and storage

81.20.-n Methods of materials synthesis and materials processing

81.16.-c Methods of nanofabrication and processing

61.46.-w Structure of nanoscale materials

Subjects

Electronics and devices

Nanoscale science and low-D systems

Condensed matter: structural, mechanical & thermal

Dates

Issue 50 (16 December 2009)

Received 1 July 2009, in final form 13 October 2009

Published 12 November 2009



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