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Blue, green, and red emission from undoped and doped ZnGa2O4 colloidal nanocrystals

Ho-June Byun, Jong-Uk Kim and Heesun Yang

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Undoped, Tb3+- and Eu3+-doped ZnGa2O4 colloidal nanocrystals were synthesized by a nonhydrolytic hot solution chemistry. Undoped nanocrystals exhibited an intrinsic blue emission peaking at 437 nm by self-activated transition. The emissions of Tb3+-and Eu3+-doped ZnGa2O4 nanocrystals consisted of their own characteristic green and red line peaks (5D47Fj transitions), respectively. Synthetic parameters such as activator concentration and reaction time were varied to investigate their effects on luminescent properties. Tb3+-doped colloidal nanocrystals synthesized for a short reaction time showed an unprecedented, exclusively green luminescence with the host blue emission effectively suppressed. On the other hand, the emission of Eu3+-doped ones was weak with the host emission persistently present regardless of reaction time.


PACS

78.67.Bf Nanocrystals and nanoparticles

82.70.Dd Colloids

61.72.up Other materials

81.16.-c Methods of nanofabrication and processing

78.55.Hx Other solid inorganic materials

Subjects

Soft matter, liquids and polymers

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Nanoscale science and low-D systems

Chemical physics and physical chemistry

Dates

Issue 49 (9 December 2009)

Received 27 July 2009, in final form 17 October 2009

Published 6 November 2009



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