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Fabrication and good ethanol sensing of biomorphic SnO2 with architecture hierarchy of butterfly wings

Fang Song1, Huilan Su1,3, Jie Han1, Di Zhang1,3 and Zhixin Chen2

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Using super-hydrophobic butterfly wings as templates, we developed an aqueous sol–gel soakage process assisted by ethanol-wetting and followed by calcination to fabricate well-organized porous hierarchical SnO2 with connective hollow interiors and thin mesoporous walls. The exquisite hierarchical architecture of SnO2 is faithfully replicated from the lightweight skeleton of butterfly wings at the level from nano- to macro-scales. On the basis of the self-assembly of SnO2 nanocrystallites with diameter around 7.0 nm, the interconnected tubes (lamellas), the fastigiated hollow tubers (pillars) and the double-layered substrates further construct the biomorphic hierarchical architecture. Benefiting from the small grain size and the unique hierarchical architecture, the biomorphic SnO2 as an ethanol sensor exhibits high sensitivity (49.8 to 50 ppm ethanol), and fast response/recovery time (11/31 s to 50 ppm ethanol) even at relatively low working temperature (170 °C).


PACS

85.85.+j Micro- and nano-electromechanical systems (MEMS/NEMS) and devices

89.60.Ec Environmental safety

82.80.-d Chemical analysis and related physical methods of analysis

81.16.Be Chemical synthesis methods

61.46.-w Structure of nanoscale materials

Subjects

Electronics and devices

Environmental and Earth science

Nanoscale science and low-D systems

Chemical physics and physical chemistry

Dates

Issue 49 (9 December 2009)

Received 15 July 2009, in final form 24 October 2009

Published 6 November 2009



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