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Study of hybrid solar cells made of multilayer nanocrystalline titania and poly(3-octylthiophene) or poly-(3-(2-methylhex-2-yl)-oxy-carbonyldithiophene)

Maria Antoniadou1, Elias Stathatos2, Nikolaos Boukos3, Andreas Stefopoulos4, Joannis Kallitsis4, Frederik C Krebs5 and Panagiotis Lianos1,6

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Hybrid solar cells have been constructed by using nanocrystalline titania and hole-transporting polymers. Titania was deposited on fluorine-doped tin-oxide transparent electrodes in three layers: a blocking layer and two nanostructured layers, giving densely packed or open structures. Open structures produced higher currents due to better polymer penetration and larger oxide–polymer interface. Cells based on the dithiophene-unit-containing polymer gave higher open-circuit voltage. Efficient cells could be made only in the presence of a dye sensitizer and a lithium salt. Cells were neither sealed nor encapsulated and their components were deposited under ambient conditions except for the metal back electrode, which was deposited under vacuum. Cells demonstrated a transient behavior in two stages: initially an increase of both current and voltage followed by an increase in voltage and a drop in current. Both quantities were stabilized at values approximately established within a few days. These values remained stable for several months when the cells were stored in the dark.


PACS

84.60.Jt Photoelectric conversion: solar cells and arrays

61.46.Hk Nanocrystals

61.41.+e Polymers, elastomers, and plastics

68.65.Ac Multilayers

73.63.Bd Nanocrystalline materials

81.16.-c Methods of nanofabrication and processing

Subjects

Soft matter, liquids and polymers

Electronics and devices

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 49 (9 December 2009)

Received 15 September 2009, in final form 19 October 2009

Published 6 November 2009



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