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Three-dimensional selective growth of nanoparticles on a polymer microstructure

Shaomin Wu1, Li-Hsin Han2 and Shaochen Chen2

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We demonstrate a new technique for selectively growing gold nanoparticles on a patterned three-dimensional (3D) polymer microstructure. The technique integrates 3D direct writing of heterogeneous microstructures with nanoparticle synthesis. A digital micromirror device is employed as a dynamic mask in the digital projection photopolymerization process to build the heterogeneous microstructure layer by layer. An amine-bearing polyelectrolyte, branched poly(ethylenimine), is selectively attached to the microstructure and acts as both a reducing and a protective agent in the nanoparticle synthesis. Scanning electron microscopy, energy dispersive x-ray spectroscopy and x-ray photoelectron spectroscopy are utilized to analyze the microstructure and the 3D selectivity of the nanoparticle growth.


PACS

81.07.Bc Nanocrystalline materials

82.80.Ej X-ray, Mössbauer, and other gamma-ray spectroscopic analysis methods

79.60.Jv Interfaces; heterostructures; nanostructures

81.16.Rf Nanoscale pattern formation

82.35.Rs Polyelectrolytes

61.46.Df Structure of nanocrystals and nanoparticles ("colloidal" quantum dots but not gate-isolated embedded quantum dots)

Subjects

Soft matter, liquids and polymers

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Biological physics

Nanoscale science and low-D systems

Chemical physics and physical chemistry

Dates

Issue 28 (15 July 2009)

Received 22 February 2009, in final form 10 May 2009

Published 23 June 2009



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