Quick search Find article
Quick search
Find article

Solvent-dependent fluorescence property of multi-walled carbon nanotubes noncovalently functionalized by pyrene-derivatized polymer

Yan Gao1,2,3, Minmin Shi2,3, Renjia Zhou1,2,3, Chaohua Xue2,3, Mang Wang2,3 and Hongzheng Chen1,2,3,4

Show affiliations


Multi-walled carbon nanotubes (MWCNTs) were supramolecularly functionalized by pyrene-derivatized hydrolyzed poly(styrene-co-maleic anhydride) (pyrene–HSMA) in aqueous solution. The MWCNTs/pyrene–HSMA conjugates were found to exhibit a solvent-dependent fluorescence property by photoluminescence measurements. The fluorescence intensity of the MWCNTs/pyrene–HSMA conjugate was used as a probe to estimate the interaction between polymer and MWCNTs in solvents. The polymer conformation around the MWCNTs was demonstrated by atomic force microscopy. We suggested that pyrene–HSMA functionalized MWCNTs in a non-wrapping mode, and that the conformation change of the polymer around the MWCNTs resulted in the solvent-dependent fluorescence property. The dispersion state of the MWCNTs/pyrene–HSMA conjugate in various solvents was also investigated by transmission electron microscopy. The fluorescence responses of the MWCNTs/pyrene–HSMA conjugate to pH value and temperature were studied as well.


PACS

78.67.Ch Nanotubes

68.37.Lp Transmission electron microscopy (TEM)

68.37.Ps Atomic force microscopy (AFM)

78.55.Hx Other solid inorganic materials

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 13 (1 April 2009)

Received 28 November 2008, in final form 26 January 2009

Published 11 March 2009



View by subject




Export








Please login to access our web services, or create an account if you don't yet have one.

You must have cookies enabled in your web browser to be able to login.

Username
Password

Forgotten your password? Get a new one here.