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Imaging buried organic islands by spatially resolved ballistic electron emission spectroscopy

Kuan Eng J Goh, A Bannani1 and C Troadec

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The well-known Au/n-Si(111) Schottky interface is modified by a discontinuous pentacene film (~1.5 nm thick) and studied using spatially resolved ballistic electron emission spectroscopy (BEES). The pentacene film introduced subtle changes to the interface which cannot be definitively detected by current–voltage measurements or a standard BEES analysis of the barrier height. In contrast, analyzing the BEES results in a dual-parameter (transmission attenuation and barrier height) space allows the effect of the pentacene film on the Au/n-Si(111) interface to be clearly demonstrated. We found that the pentacene film behaves like a tunneling barrier and increases the distribution of local barrier heights with a tendency toward lower values. Our results highlight the potential of the dual-parameter BEES analysis for understanding local interface modification by molecules.


PACS

73.30.+y Surface double layers, Schottky barriers, and work functions

73.40.Qv Metal-insulator-semiconductor structures (including semiconductor-to-insulator)

Subjects

Semiconductors

Surfaces, interfaces and thin films

Dates

Issue 44 (5 November 2008)

Received 21 June 2008, in final form 3 September 2008

Published 2 October 2008



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