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A nonlinear system model for electrospinning sub-100 nm polyacrylonitrile fibres

M A Costolo, J D Lennhoff, R Pawle, E A Rietman1 and A E Stevens

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Solutions of polyacrylonitrile (PAN) were electrospun using a range of process parameters, resulting in fibre diameters from 10 to 320 nm. A nonlinear neural network system model was used to analyse the dependence of the fibre diameter on the process parameters, and used to simulate conditions for electrospinning 40–60 nm diameter fibres. These results indicated that flow rate is most important for determining fibre diameter. It was not possible to find the appropriate conditions for electrospinning sub-25 nm fibres. Precise control of the ambient temperature and relative humidity will be critical to producing electrospun fibres that are sub-25 nm. Further, it is unlikely that sub-25 nm fibres will be produced without significant changes in the electrospinning apparatus, for example, by use of focusing and jet-steering fields, alternate carrier gases to modify the discharge characteristics, or patterned electrospinning.


PACS

81.16.-c Methods of nanofabrication and processing

81.07.-b Nanoscale materials and structures: fabrication and characterization

Subjects

Nanoscale science and low-D systems

Dates

Issue 3 (23 January 2008)

Received 21 June 2007, in final form 15 November 2007

Published 13 December 2007



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