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The microstructure and electrical conductivity of mixed-valence TlIn4S5Cl quaternary compound micro- and nanowires

Xin Jiang1, Hans-Jörg Deiseroth2, Changzhi Gu3, Kledi Xhaxhiu2, Yang Huang3, Junjie Li3, Renchao Che3 and Zongli Wang3

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Quaternary mixed-valence compound TlIn4S5Cl micro- and nanowires are prepared by partial substitution of chalcogen with halogen starting from a stoichiometric mixture of TlCl, In and S. Their electrical conductivity and gas sensitivity properties are investigated by using standard four-terminal systems. The specific nanowire resistivity is about 107 Ω cm and corresponds to the value of a typical undoped semiconductor in air. This resistivity is, however, extremely sensitive to NO2 (sensitivity about 150) or NH3, with a rapid response of about 2 s and recovery times. This phenomenon is supposed to be particularly important for future nanodevice applications.


PACS

73.63.-b Electronic transport in nanoscale materials and structures

81.16.-c Methods of nanofabrication and processing

68.65.-k Low-dimensional, mesoscopic, and nanoscale systems: structure and nonelectronic properties

Subjects

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 20 (21 May 2008)

Received 13 December 2007, in final form 11 March 2008

Published 15 April 2008



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