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Functionalization of BN nanotubes with dichlorocarbenes

Yafei Li1, Zhen Zhou1 and Jijun Zhao2

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The geometric and electronic structures of dichlorocarbene (CCl2) functionalized BN nanotubes (BNNTs) were studied using density functional theory within the generalized gradient approximation. We found that the CCl2 addition favors slanted B–N bonds in zigzag tubes, and the CCl2-attached BNNTs prefer open rather than closed three-membered-ring (3MR) structures in all the zigzag (n,0) BNNTs studied, whereas closed 3MR structure occurs in the CCl2-attached BN graphene layer. The binding energies decrease with increase of the CCl2 coverage, but the electronic properties of BNNTs do not change significantly, irrespective of the CCl2 coverage.


PACS

61.46.Fg Nanotubes

71.15.Mb Density functional theory, local density approximation, gradient and other corrections

71.15.Nc Total energy and cohesive energy calculations

73.22.-f Electronic structure of nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals

Subjects

Condensed matter: electrical, magnetic and optical

Nanoscale science and low-D systems

Dates

Issue 1 (9 January 2008)

Received 31 August 2007, in final form 23 October 2007

Published 29 November 2007



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