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Reverse self-assemblies based on amphiphilic polyphosphazenes for encapsulation of water-soluble molecules

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Liyan Qiu1,3, Jianxiang Zhang1,2, Meiqiu Yan1, Yi Jin1 and Kangjie Zhu2

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A novel series of amphiphilic polyphosphazenes (PNIPAm/AA-PPP) containing hydrophilic oligo-(N-isopropylacrylamide) (oligo-NIPAm) and various hydrophobic aliphatic amines as co-substitutes was synthesized via a two-step substitution reaction. The extraction and solubilization of water-soluble substances such as fluorescein sodium and trypan blue from an aqueous phase into the chloroform phase were supposed to result from the formation of polyphosphazene reverse self-assemblies in the organic phase. A field emission scanning electronic microscope was adopted to characterize the morphology of reverse assemblies in chloroform. Additionally, a significant improvement of encapsulation and release profiles of water-soluble substances was found for poly(lactic-co-glycolic acid) (PLGA) microparticles in the presence of amphiphilic copolymers, which was associated with the chemical structure of copolymers as well as the content of copolymer in the microparticles.


PACS

82.70.Uv Surfactants, micellar solutions, vesicles, lamellae, amphiphilic systems, (hydrophilic and hydrophobic interactions)

82.35.Jk Copolymers, phase transitions, structure

64.75.-g Phase equilibria

81.16.Dn Self-assembly

Subjects

Soft matter, liquids and polymers

Nanoscale science and low-D systems

Chemical physics and physical chemistry

Dates

Issue 47 (28 November 2007)

Received 1 August 2007, in final form 6 September 2007

Published 19 October 2007



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