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Copper indium diselenide nanowire arrays by electrodeposition in porous alumina templates

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Sovannary Phok, Suresh Rajaputra and Vijay P Singh

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A simple template assisted approach for fabricating I–III–VI semiconductor nanowire arrays is presented. Vertically aligned arrays of CuInSe2 (CIS) nanowires of controllable diameter and length were synthesized by pulse cathodic electrodeposition from a novel acidic electrolyte solution into anodized alumina (AAO) templates, followed by annealing at 220 °C in vacuum. Scanning electron microscopy revealed that the nanowires were dense and compact. Depending on the dimensions of the starting AAO template, the diameters ranged from 5 to 40 nm and the lengths ranged from 600 nm to 5 µm; the grain size was estimated to be less than 5 nm. The composition of the nanowires was analyzed by energy dispersive x-ray (EDX) spectroscopy, and was found to be close to stoichiometric CuInSe2 within the limit of the resolution of the EDX technique. High resolution transmission electron microscopy and x-ray diffraction revealed high purity CuInSe2 nanowires with a preferred [112] orientation.


PACS

61.46.-w Structure of nanoscale materials

82.45.Qr Electrodeposition and electrodissolution

81.16.-c Methods of nanofabrication and processing

81.07.-b Nanoscale materials and structures: fabrication and characterization

82.45.Yz Nanostructured materials in electrochemistry

Subjects

Nanoscale science and low-D systems

Chemical physics and physical chemistry

Dates

Issue 47 (28 November 2007)

Received 17 July 2007, in final form 21 September 2007

Published 17 October 2007



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