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Ultrafast dynamics in ZnO/ZnMgO multiple quantum wells

X M Wen1,2, J A Davis2, D McDonald2, L V Dao2, P Hannaford2, V A Coleman3, H H Tan3, C Jagadish3, K Koike4, S Sasa4, M Inoue4 and M Yano4

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We have investigated carrier relaxation and exciton recombination dynamics in ZnO/ZnMgO multiple quantum wells using femtosecond pump–probe techniques at room temperature. For a probe energy above the band gap, the hot carriers exhibit an effective relaxation by longitudinal optical phonon scattering with a cooling time of 700–850 fs. By detecting the emission near the band-gap, a longer decay time of a few picoseconds was observed which is attributed to acoustic phonon scattering. As the probe energy is decreased further, the decay time continues to increase due to the transitions of exciton recombination or localized carrier recombination.


PACS

73.63.Hs Quantum wells

72.20.Jv Charge carriers: generation, recombination, lifetime, and trapping

73.20.Mf Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)

78.67.De Quantum wells

73.21.Fg Quantum wells

Subjects

Condensed matter: electrical, magnetic and optical

Semiconductors

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 31 (8 August 2007)

Received 22 April 2007, in final form 14 June 2007

Published 6 July 2007



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