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Polyhedral oligomeric silsequioxane monolayer as a nanoporous interlayer for preparation of low-k dielectric films

Ying-Ling Liu1,3, Chuan-Shun Liu1, Chin-I Cho1 and Ming-Jyh Hwu2

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Polyhedral oligomeric silsequioxane (POSS) monomer was fixed to a silicon surface by reacting octakis(glycidyldimethylsiloxy)octasilsesquioxane (OG-POSS) with the OH-terminated silicon surface in the presence of tin (II) chloride. The POSS cage layer then served as a nanoporous interlayer to reduce the dielectric constants of polyimide films on silicon surfaces. The chemical structure and surface morphology of OG-POSS modified silicon surfaces were characterized with XPS. With the introduction of a POSS nanopored interlayer, the dielectric constants of polyimide films were reduced.


PACS

77.55.+f Dielectric thin films

68.35.B- Structure of clean surfaces (and surface reconstruction)

68.47.Fg Semiconductor surfaces

77.22.Ch Permittivity (dielectric function)

79.60.Jv Interfaces; heterostructures; nanostructures

68.55.A- Nucleation and growth

Subjects

Condensed matter: electrical, magnetic and optical

Semiconductors

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 22 (6 June 2007)

Received 21 December 2006, in final form 11 April 2007

Published 4 May 2007



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