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Large scale continuous synthesis of carbon-encapsulated magnetic nanoparticles

M Bystrzejewski1,5, A Huczko1, H Lange1, P Baranowski1, G Cota-Sanchez2,3, G Soucy2, J Szczytko4 and A Twardowski4

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Fe, Fe3C and NdC2 nanoparticles, encapsulated within carbon cages, were continuously produced during the induction thermal plasma processing of Fe14Nd2B, in the presence of methane or acetylene. The product morphology was studied by means of SEM. Further structural details were obtained from TEM, HRTEM, Raman spectroscopy and x-ray powder diffraction studies. The so-produced nanostructures have core–shell structure, with inner cavity diameters varying between 10 and 30 nm. The carbon coatings were composed of between 5 and 25 graphene layers. The carbon cages were built from sp2 carbon atoms, which protected the encapsulated nanoparticles from both oxidation and agglomeration. The plasma generated products were ferromagnetic, with maximum values of coercivity field of 600 G s, and saturation magnetization values of up to 40 emu g−1.


PACS

81.07.Bc Nanocrystalline materials

75.60.Ej Magnetization curves, hysteresis, Barkhausen and related effects

78.30.-j Infrared and Raman spectra

75.75.+a Magnetic properties of nanostructures

61.46.Df Structure of nanocrystals and nanoparticles ("colloidal" quantum dots but not gate-isolated embedded quantum dots)

68.37.Lp Transmission electron microscopy (TEM)

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 14 (11 April 2007)

Received 7 December 2006, in final form 29 January 2007

Published 6 March 2007



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