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Instability of Ag nanoparticles in SiO2 at ambient conditions

Matthias Hillenkamp, Giulia Di Domenicantonio, Olivier Eugster and Christian Félix

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The room-temperature stability of nanometre-sized silver clusters in silica matrices has been investigated by following the temporal evolution of their surface plasmon absorption. Ag clusters in SiO2 were prepared by either annealing silica samples doped with atomic silver or by co-deposition of preformed clusters of defined size. Clusters were found to be unstable at ambient conditions on a timescale of days to weeks, independent of preparation conditions. The disappearance of the plasmonic resonance is explained by successive oxidation of the clusters even inside the matrix.


PACS

61.46.Df Structure of nanocrystals and nanoparticles ("colloidal" quantum dots but not gate-isolated embedded quantum dots)

73.21.-b Electron states and collective excitations in multilayers, quantum wells, mesoscopic, and nanoscale systems

61.46.Bc Structure of clusters (e.g., metcars; not fragments of crystals; free or loosely aggregated or loosely attached to a substrate)

Subjects

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 1 (10 January 2007)

Received 16 October 2006, in final form 6 November 2006

Published 8 December 2006



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