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Stable luminescent films and hollow spheres comprising CdTe nanoparticles

Z H Yang, L L Yang, S Bai, Z F Zhang and W X Cao1

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CdTe nanoparticles (CdTe-NPs) capped by 3-mercaptopropionic acid were synthesized and used to self-assemble (SA) with poly(allylamine hydrochloride) (PAH) layer-by-layer via electrostatic interaction to form luminescent multilayer films. Composite particles were prepared with polymer or SiO2 beads as the core and PAH/CdTe-NP SA films as the shell. The composite particles were dissolved out of the core with tetrahydrofuran (THF) or HF to prepare hollow spheres, then treated with 1-ethyl-3-(3-dimethyl-aminopropyl)-carbodiimide hydrochloride (EDC) in aqueous solution to form stable hollow spheres with a crosslinked PAH/CdTe-NP shell. Both the crosslinked films and the hollow spheres with a high luminescence are very stable in aqueous solutions at a wide range of pH.


PACS

81.07.Wx Nanopowders

78.60.Fi Electroluminescence

81.16.Dn Self-assembly

81.16.Be Chemical synthesis methods

78.67.Pt Multilayers; superlattices

68.55.A- Nucleation and growth

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 8 (28 April 2006)

Received 6 September 2005, in final form 13 December 2005

Published 15 March 2006



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