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Large-scale production of carbon-coated copper nanoparticles for sensor applications

E K Athanassiou, R N Grass and W J Stark

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Copper nanoparticles with a mean carbon coating of about 1 nm were continuously produced at up to 10 g h−1 using a modified flame spray synthesis unit under highly reducing conditions. Raman spectroscopy and solid state 13C magic angle spinning nuclear magnetic resonance spectroscopy revealed that the thin carbon layer consisted of a sp2-hybridized carbon modification in the form of graphene stacks. The carbon layer protected the copper nanoparticles from oxidation in air. Bulk pills of pressed carbon/copper nanoparticles displayed a highly pressure- and temperature-dependent electrical conductivity with sensitivity at least comparable to commercial materials. These properties suggest the use of thin carbon/copper nanocomposites as novel, low-cost sensor materials and offer a metal-based alternative to the currently used brittle oxidic spinels or perovskites.


PACS

61.46.Df Structure of nanocrystals and nanoparticles ("colloidal" quantum dots but not gate-isolated embedded quantum dots)

73.63.-b Electronic transport in nanoscale materials and structures

78.30.Er Solid metals and alloys

68.37.Lp Transmission electron microscopy (TEM)

76.60.-k Nuclear magnetic resonance and relaxation

61.05.cp X-ray diffraction

07.07.Df Sensors (chemical, optical, electrical, movement, gas, etc.); remote sensing

Subjects

Condensed matter: electrical, magnetic and optical

Instrumentation and measurement

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 6 (28 March 2006)

Received 9 January 2006, in final form 30 January 2006

Published 27 February 2006



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