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Characterization of crystalline dendrimer-stabilized gold nanoparticles

Xiangyang Shi1, T Rose Ganser1, Kai Sun2, Lajos P Balogh1 and James R Baker Jr1

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Monodispersed, highly crystalline dendrimer-stabilized gold nanoparticles (Au DSNPs) were synthesized via hydrazine reduction chemistry and stabilized using primary amine-terminated poly(amidoamine) (PAMAM) dendrimers of different generations (generations 2–6) with the same molar ratios of dendrimer terminal nitrogen ligands/gold atoms. The sizes of the synthesized Au DSNPs decrease with the increase of the number of dendrimer generations. These Au DSNPs are fluorescent and display strong blue emission intensity at 458 nm. Polyacrylamide gel electrophoresis (PAGE) analysis indicates that all Au DSNPs are stable and both metal NPs and dendrimer stabilizers do not separate from each other during the electrophoresis process. The synthesized inorganic/organic hybrid Au DSNPs provide new nanoplatforms that will be further modified with various biological ligands for the application of biosensing and targeted cancer therapeutics.


PACS

81.07.Pr Organic-inorganic hybrid nanostructures

82.45.Yz Nanostructured materials in electrochemistry

78.67.Bf Nanocrystals and nanoparticles

68.70.+w Whiskers and dendrites (growth, structure, and nonelectronic properties)

81.07.Wx Nanopowders

81.16.Be Chemical synthesis methods

Subjects

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Chemical physics and physical chemistry

Dates

Issue 4 (28 February 2006)

Received 12 October 2005, in final form 13 December 2005

Published 30 January 2006



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