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Electrostatic force spectroscopy of near surface localized states

Aykutlu Dâna1 and Yoshihisa Yamamoto2

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Electrostatic force microscopy at cryogenic temperatures is used to probe the electrostatic interaction of a conductive atomic force microscopy tip and electronic charges trapped in localized states in an insulating layer on a semiconductor. Measurement of the frequency shift of the cantilever as a function of tip–sample bias voltage shows discrete peaks at certain voltages when the tip is located near trap centres. These discrete changes in frequency are attributed to one by one filling of individual electronic states when the quantized energies traverse the substrate conduction band Fermi energy as the tip–sample voltage is increased. Theoretical analysis of the experiment suggests that such a measurement of the cantilever frequency shift as a function of bias voltage can be interpreted as an AC force measurement, from which spectroscopic information about the location and energy of localized states can be deduced. Experimental results from the study of a sample with InAs quantum dots as trap centres are presented.


PACS

73.20.Fz Weak or Anderson localization

73.21.La Quantum dots

73.50.Gr Charge carriers: generation, recombination, lifetime, trapping, mean free paths

73.63.Kv Quantum dots

73.20.At Surface states, band structure, electron density of states

Subjects

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Dates

Issue 3 (March 2005)

Received 30 September 2004, in final form 14 January 2005

Published 3 February 2005



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