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Large-scale synthesis and field emission properties of vertically oriented CuO nanowire films

Y W Zhu1,2, T Yu1, F C Cheong1, X J Xu3,4, C T Lim3,4, V B C Tan3,4, J T L Thong3,5 and C H Sow1,2,6

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Using a simple method of direct heating of bulk copper plates in air, oriented CuO nanowire films were synthesized on a large scale. The length and density of nanowires could be controlled by growth temperature and growth time. Field emission (FE) measurements of CuO nanowire films show that they have a low turn-on field of 3.5–4.5 V µm−1 and a large current density of 0.45 mA cm−2 under an applied field of about 7 V µm−1. By comparing the FE properties of two types of samples with different average lengths and densities (30 µm, 108 cm−2 and 4 µm, 4 × 107 cm−2, respectively), we found that the large length–radius ratio of CuO nanowires effectively improved the local field, which was beneficial to field emission. Verified with finite element calculation, the work function of oriented CuO nanowire films was estimated to be 2.5–2.8 eV.


PACS

79.70.+q Field emission, ionization, evaporation, and desorption

81.20.-n Methods of materials synthesis and materials processing

68.55.-a Thin film structure and morphology

81.07.-b Nanoscale materials and structures: fabrication and characterization

73.30.+y Surface double layers, Schottky barriers, and work functions

61.46.-w Structure of nanoscale materials

Subjects

Condensed matter: electrical, magnetic and optical

Surfaces, interfaces and thin films

Nanoscale science and low-D systems

Condensed matter: structural, mechanical & thermal

Dates

Issue 1 (January 2005)

Received 25 August 2004, in final form 19 October 2004

Published 2 December 2004



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