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The viability of 0.3 nm diameter carbon nanotubes

Y L Mao1, X H Yan1,2,3, Y Xiao1, J Xiang1, Y R Yang1 and H L Yu1

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Using first-principles calculations, we investigate the comparative stability of sub-0.4 nm carbon nanotubes. Compared to the fullerenes C20 and C60, it is found that the most likely carbon nanotubes with a small diameter 0.3 nm are (2,2),(3,1) and (4,0) nanotubes. The spontaneous symmetry breaking of an isolated (2,2) nanotube produces an energy gap at the Fermi level converting it into a semiconductor. The curvature effects lowered the π* band to cross the Fermi energy, leading to the (4,0) nanotube being metallic.


PACS

73.22.-f Electronic structure of nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals

71.15.-m Methods of electronic structure calculations

Subjects

Condensed matter: electrical, magnetic and optical

Nanoscale science and low-D systems

Dates

Issue 8 (August 2004)

Received 12 January 2004

Published 18 June 2004



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