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Conformational study of porphyrin-based molecules using non-contact atomic force microscopy

Shukichi Tanaka, Hitoshi Suzuki, Toshiya Kamikado and Shinro Mashiko

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To control the interaction between tetrakis(3,5 di-t-butylphenyl)porphyrin (TBPP) molecules and substrates, 5-(4-methylthiophenyl)-10,15,20-tris(3,5-di-t-butylphenyl)porphyrin (MSTBPP) molecules were tailored; one of the four di-t-butylphenyl groups of TBPP molecules was replaced by a methylthiophenyl group. By means of non-contact atomic force microscopy (NC-AFM) operated in the force feedback control mode, the conformation of MSTBPP molecules deposited on an Au(111) substrate was investigated. It was found that the methylthiophenyl group introduced into the TBPP molecules enhanced the attractive interaction between the molecule and the substrate. This interaction seems to improve the spatial resolution of NC-AFM.


PACS

37.10.De Atom cooling methods

33.15.Bh General molecular conformation and symmetry; stereochemistry

Subjects

Atomic and molecular physics

Dates

Issue 2 (February 2004)

Received 26 August 2003, in final form 19 December 2003

Published 22 January 2004



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