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High-concentration nitrogen-doped carbon nanotube arrays

L M Cao1,4, X Y Zhang2, C X Gao1, W K Wang1,2, Z L Zhang3 and Z Zhang3

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Large arrays of aligned CNx nanotubes were synthesized by radiofrequency magnetron sputtering of a mixture of nanometre-sized graphite and nickel powders in a nitrogen atmosphere. The CNx nanotubes produced assembled into bundle-like arrays standing perpendicularly on the silicon substrates. The nickel nanoparticles located in the tips suggest that a 'tip-growth' mechanism governs their growth process. Transmission electron microscopy and electron energy-loss spectroscopy studies reveal that the nanotubes possess a bamboo-like structure and nitrogen to carbon atomic ratios in the range of 0.22–0.32, commensurate with C3Nx (x < 1) stoichiometries. Our results illustrate the potential of the magnetron sputtering method for the creation of a large number of ordered nanostructures.


PACS

81.07.De Nanotubes

61.46.-w Structure of nanoscale materials

81.16.Dn Self-assembly

61.50.Nw Crystal stoichiometry

68.47.Fg Semiconductor surfaces

Subjects

Semiconductors

Surfaces, interfaces and thin films

Condensed matter: structural, mechanical & thermal

Nanoscale science and low-D systems

Dates

Issue 8 (August 2003)

Received 9 March 2003, in final form 9 June 2003

Published 2 July 2003



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