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Effect of iron additions on intergranular cohesion in chromium

T Ossowski, E Wachowicz and A Kiejna

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The structural, cohesive, and magnetic properties of (111) and (210) tilt grain boundaries (GBs) in pure Cr, and in Cr with Fe additions, are studied from first principles. Different concentration and position of solute atoms are considered. Our calculations show that Fe atoms placed in the GB interstice enhance cohesion, whereas Fe substituted for one of the Cr layer atoms, in most cases, has very small (or negligible) effect on the cohesion at GBs in Cr. We have found that Fe additions show a tendency to enrich the boundaries in Cr. In the presence of Fe additions the magnetic moments on the GB host atoms are substantially modified and those on Fe impurities are reduced. In most cases the moments on Fe additions remain much higher than the local moments on the Cr atoms.


PACS

61.72.Mm Grain and twin boundaries

75.30.Hx Magnetic impurity interactions

75.50.Ee Antiferromagnetics

75.50.Bb Fe and its alloys

75.30.Cr Saturation moments and magnetic susceptibilities

Subjects

Condensed matter: electrical, magnetic and optical

Condensed matter: structural, mechanical & thermal

Dates

Issue 48 (2 December 2009)

Received 26 June 2009, in final form 4 September 2009

Published 30 October 2009



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