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Heterogeneous nucleation and growth of the β(Ti) phase in the Ti–Al system—experiments and model calculations

Daniel Gosslar1, Christian Hartig1, Robert Günther1, Ulrike Hecht2 and Rüdiger Bormann1

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The barrier to heterogeneous nucleation of the β(Ti) phase on TiB2 and other borides has been evaluated using the plane to plane matching model. The results are compared to the known nucleation of the α(Ti) phase on the β(Ti) phase. According to this comparison, the barrier to heterogeneous nucleation of the β(Ti) phase on TiB2 can be judged to be small. This is in agreement with inoculation experiments. The addition of a Ti–Al–TiB2 master composite to a β(Ti) solidifying TiAl based alloy leads to a significantly refined microstructure. Microsegregations enable us to attribute this refinement to refined equiaxed β(Ti) dendrites. However, model calculations based on the hemispherical cap model predict that the refinement via heterogeneous β(Ti) nucleation should be more potent. First calculations indicate that structural imperfections of TiB2 particles limit the nucleation site diameter. Thereby, the nucleation barrier is increased and the refinement is less pronounced.


PACS

64.60.Q- Nucleation

68.70.+w Whiskers and dendrites (growth, structure, and nonelectronic properties)

81.30.Fb Solidification

64.70.D- Solid–liquid transitions

64.75.-g Phase equilibria

Subjects

Soft matter, liquids and polymers

Surfaces, interfaces and thin films

Condensed matter: structural, mechanical & thermal

Dates

Issue 46 (18 November 2009)

Received 22 April 2009

Published 27 October 2009



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