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Temperature evolution of the magnetic excitations in charge ordered La5/3Sr1/3NiO4

P G Freeman1, A T Boothroyd2, R A Ewings2, M Hücker3, D Prabhakaran2, M Enderle1 and J M Tranquada3

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Polarized- and unpolarized-neutron scattering was used to study the temperature evolution of the magnetic excitations of charge ordered La5/3Sr1/3NiO4. We studied two features in detail: (i) the resonance-like scattering at 27 meV in the quasi-two-dimensional magnetic excitations from the ordered Ni2+ (S = 1) spins, and (ii) the diffuse scattering associated with quasi-one-dimensional antiferromagnetic correlations along the stripes. Although both these features persist up to at least ~125 K, their temperature dependences are found to be quite different. We argue from the results that the resonance-like feature observed in La2−xSrxNiO4 (x~1/3) is not caused by a coupling between the spin dynamics of the two magnetic sub-systems.


PACS

75.25.+z Spin arrangements in magnetically ordered materials (including neutron and spin-polarized electron studies, synchrotron-source x-ray scattering, etc.)

75.50.Ee Antiferromagnetics

Subjects

Condensed matter: electrical, magnetic and optical

Dates

Issue 10 (12 March 2008)

Received 11 July 2007, in final form 5 October 2007

Published 19 February 2008



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